Dynamic Assembly and Functions of Surfactants★

doi:10.6023/A26060189

Acta Chimica Sinica ›› 2026, Vol. 84 ›› Issue (8): 1365-1375.DOI: 10.6023/A26060189 Previous Articles Next Articles

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表面活性剂的动态组装与功能^★

张紫祺^a^,^b, 范雅珣^a^,^b^,^*(), 王毅琳^a^,^b^,^*()

^a 中国科学技术大学化学与材料科学学院仿生界面材料科学全国重点实验室合肥 230026
² 中国科学技术大学苏州高等研究院纳米科学技术学院仿生界面材料科学全国重点实验室苏州 215123

投稿日期:2026-06-09 发布日期:2026-08-12
通讯作者: 范雅珣, 王毅琳

作者简介:

张紫祺, 2021年毕业于兰州大学化学与化工学院, 随后加入中国科学院化学研究所王毅琳研究员课题组, 于2026年获得物理化学博士学位, 主要从事调控表面活性剂聚集体对农药吸收传导的影响和微生物农药包封性能的研究.

王毅琳, 1988和1991年分别在兰州大学获学士和硕士学位; 1991~1994年在兰州大学任讲师; 1997年在中国科学院化学研究所获博士学位; 1997~2001年, 先后在美国佛罗里达大学和印第安那-普渡大学进行博士后工作; 2002~2024年, 任中国科学院化学研究所研究员; 2014~2024年, 兼任中国科学院大学岗位教授; 2025年1月起, 作为讲席教授就职于中国科学技术大学, 在中国科学技术大学苏州高等研究院工作. 曾入选中国科学院“百人计划”, 获国家杰出青年科学基金, 并获中国化学会胶体与界面杰出贡献奖等荣誉, 目前作为项目负责人承担国家重点研发计划项目, 担任Langmuir的执行主编、Curr. Opin. Colloid Interface Sci.表面活性剂部分的主编、以及《化学学报》、Soft Matter、Colloid Surf., A及ACS Omega等期刊的编委. 长期从事以溶液中表面活性剂为核心的基础和应用研究, 发展了表面活性剂在提高农药利用率、个人护理、杀菌及工业清洗等方面的功能.

^★“纪念兰州大学化学学科创建80周年”专辑

基金资助:
国家重点研发计划(2021YFA0716700); 苏州市科技计划项目(ZXP2025309); 苏州市科技计划项目(ZXP2025067); 苏州仿生界面科学重点实验室(SZ2024004)

Dynamic Assembly and Functions of Surfactants^★

Ziqi Zhang^a^,^b, Yaxun Fan^a^,^b^,^*(), Yilin Wang^a^,^b^,^*()

^a State Key Laboratory of Bioinspired Interfacial Materials Science, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei 230026, China
² State Key Laboratory of Bioinspired Interfacial Materials Science, and School of Nano Science and Technology, Suzhou Institute for Advanced Research, University of Science and Technology of China, Suzhou 215123, China

Received:2026-06-09 Published:2026-08-12
Contact: Yaxun Fan, Yilin Wang
About author:
^★For the VSI “Celebration of 80th Anniversary of Chemistry in Lanzhou University”
Supported by:
National Key Research and Development Program of China(2021YFA0716700); Science and Technology Project of Suzhou(ZXP2025309); Science and Technology Project of Suzhou(ZXP2025067); Suzhou Key Laboratory of Bioinspired Interfacial Materials Science(SZ2024004)

Surfactants, owing to their unique amphiphilic nature and excellent interfacial activity, have been widely applied in household chemicals, cleaning, food processing, medicine, agriculture, and petroleum recovery. However, conventional surfactants often suffer from low utilization efficiency, environmental contamination, and limited functionality during practical applications, creating an urgent demand for the development of highly efficient, environmentally friendly, and multifunctional surfactant systems. Recent studies have demonstrated that the dynamic assembly behavior of surfactants at interfaces and in bulk solution plays a decisive role in their practical performance. By regulating surfactant molecular structures, aggregate morphologies, and dynamic transformation processes, the interfacial behaviors and functional properties of surfactant systems can be precisely controlled. Recent advances in the dynamic assembly and functional applications of surfactants, including low-foaming and highly efficient cleaning, long-lasting antibacterial activity, enhanced boiling heat transfer of droplets impacting overheated surfaces, suppression of Worthington jets generated by droplet impact on liquid pools and promotion of efficient deposition and spreading of pesticide droplets on superhydrophobic crop surfaces, are systematically summarized. Particular emphasis is placed on the critical roles of hierarchical assemblies, such as vesicles, wormlike micelles, and coacervates, in interfacial migration, structural transformation, and functional realization. Finally, the future prospects of dynamically assembled surfactant systems in green cleaning, efficient heat transfer, precision agriculture, and smart responsive materials are discussed, aiming to provide guidance for the design and practical applications of next-generation functional surfactant systems.

Key words: surfactant, dynamic assembly, low-foam cleaning, efficient sterilization, droplet impact

Cite this article

Ziqi Zhang, Yaxun Fan, Yilin Wang. Dynamic Assembly and Functions of Surfactants^★[J]. Acta Chimica Sinica, 2026, 84(8): 1365-1375.

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Fig. & Tab. 6

Figure 1. Construction of low-foaming and recyclable cleaning surfactant systems: (a) Chemical structure, oil removal efficiency, foaming properties and foam stability of different sulfonate surfactants[44]; (b) Possible mechanism of the decay process for foams in single SDS solution and CnN/SDS (n=6, 8 and 12) solution[45]; (c) Schematic diagram for high-efficiency oil-fouling removal strategy[46]

Figure 2. Highly efficient antibacterial performance of surfactants: (a) Schematic graph of antibacterial mechanism of the surfactant micelles to E. coli[58]; (b) Schematic graph of the antibacterial mechanism of peptide amphiphiles 12-(Lys)n-12 with varying spacer lengths[59]; (c) path of the molecular assembly of GA and 12-3-12 to form aggregates and the antibacterial effect of the modified coating after being soaked for 30 d[61]

Figure 3. Evaporation states and evaporation rate curves of pure water droplets and surfactant droplets impact the superheated surfaces as a function of surface temperature[75]

Figure 4. Partition diagram of jet models with the difference between the dynamic surface tension and static surface tension (Δγ=γ12 ms-γs) as the y-axis, and γ60 ms as the x-axis[83]

Figure 5. Inhibition of rebound and splash of high-speed impact droplets on superhydrophobic surfaces by surfactant aggregates: (a) Molecular structure of single-head double-tail surfactant, Cryo-TEM image of formed vesicles, behavior of droplets after impacting the superhydrophobic surface, and schematic diagram of efficient deposition and controllable penetration of different vesicles after high-speed impact on the superhydrophobic surface[103]; (b) Molecular structures of non-covalently constructed (triamine/SDS) and covalently constructed surfactant (12-3-12-3-12), impact behavior on the superhydrophobic surface, and schematic diagram of the mechanism of efficient deposition and spreading[104]

Figure 6. Control of the entire journey of pesticide application through coacervate: (a) Schematic diagram of bottom-up spraying and deposition effects of NaDC/DXAB, NaC/DXAB, water and commercial agricultural adjuvants on the abaxial side of tomato leaves[115]; (b) chemical structure of pesticides and TIS10, Cryo-SEM images of the entanglement between coacervate droplets and the micro/nano hierarchical structures on the cabbage surface, and the process of the gradual release of dyes from the coacervate droplets with the change of pH[116]; (c) Schematic diagram of the coacervate formed by sodium lignosulfonate (SL) and cationic surfactants [DTAB, hexamethylene-1,6-bis(dodecyldimethylammonium bromide) (12-6-12) and 1,4-bis(dodecyl N,N-dimethylammonium bromide)-2,3-butanediol (12-4(OH)2-12)], SEM images and water contact angles of the superhydrophobic lotus leaf and wheat leaf surfaces, images of SL solution and coacervate droplets sprayed on the lotus leaf and wheat leaf inclined at 10°, and optical images of broad bean stomata after spraying water, SL solution, and SL/DTAB condensed phase (all containing 10 μmol/L abscisic acid) under light conditions[121]

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表面活性剂的动态组装与功能^★

Dynamic Assembly and Functions of Surfactants^★

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表面活性剂的动态组装与功能★

Dynamic Assembly and Functions of Surfactants★

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Abstract

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Fig. & Tab. 6

References 121

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表面活性剂的动态组装与功能^★

Dynamic Assembly and Functions of Surfactants^★