Synthesis Progress of Layered TMOC-based Intercalation Structures
Received date: 2015-05-14
Online published: 2015-07-17
Supported by
Project supported by the the National Basic Research Program of China (2014CB848900), the National Natural Science Foundation of China (U1232131, 11375198), the Fundamental Research Funds for the Central Universities (WK2310000035), the Recruitment Program of Global Experts and the CAS Hundred Talent Program.
Different types of intercalated agents can be in-situ intercalated into two-dimensional (2D) layered transition metal oxides and chalcogens (TMOCs), which can engineer its electronic structure at the atomic scale and tune its intrinsic physical and chemical properties (i.e. carrier concentration and mobility, magnetic, optical, and other properties). Such intercalations provide a facile way to create new types of multifunctional materials, thus largely extend 2D material's applications for opto-electronic devices, energy storage and conversion, photoelectrocatalysis, etc. Recently, many efforts have been focused on seeking suitable synthesis routes to achieve different types of intercalated nanomaterials. Here, we concisely reviewed the recent development on TMOC-based intercalations produced by various intercalated agents in-situ intercalating. The synthetic strategy of alkali metal and non-alkali metal intercalation, polymer intercalation, small organic molecules intercalation and reduced graphene oxide intercalation were mainly reviewed. Through affecting the interlayer interactions and the crystal anisotropy can realize the strategy of in-situ intercalated layered materials.
Liu Qin , Liu DaoBin , He Qun , Xiang Ting , Adnan Khalil , Song Li . Synthesis Progress of Layered TMOC-based Intercalation Structures[J]. Acta Chimica Sinica, 2015 , 73(9) : 936 -943 . DOI: 10.6023/A15050331
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