Progress of Non-Nucleophilic Electrolytes for Magnesium/Sulfur Battery
Received date: 2021-01-31
Online published: 2021-05-18
Supported by
National Natural Science Foundation of China(21773291); National Natural Science Foundation of China(U1832218); Inner Mongolia Autonomous Region Key Laboratory of Nanocarbon Materials(MDK2019008)
Non-nucleophilic magnesium electrolyte has attracted significant attention since the first non-nucleophilic organic aluminum magnesium salt with [Mg2(μ-Cl)3(THF)6]+ as the cation of electrochemical active center for magnesium/sulfur (Mg/S) cells was reported by Muldoon group in 2011. In this work, we reviewed the synthesis, cation structure and electrochemical performance of non-nucleophilic magnesium electrolyte for Mg/S battery. The future research directions of non-nucleophilic Mg/S battery electrolyte are discussed. It is pointed out that in order to promote the industrialization of Mg/S battery, in addition to the development of non-nucleophilic electrolyte materials with high performance, low cost and simple structure, further mechanistic understanding for optimization of electrolyte composition and for better matching between the electrolyte with positive or negative electrode materials is also very important.
Wanfei Li , Xin Li , Haiyan Fan , Jianhua Xiao , Qianqian Liu , Miao Cheng , Jing Hu , Tao Wei , Zhengying Wu , Yun Ling , Bo Liu , Yuegang Zhang . Progress of Non-Nucleophilic Electrolytes for Magnesium/Sulfur Battery[J]. Acta Chimica Sinica, 2021 , 79(5) : 628 -640 . DOI: 10.6023/A21010038
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