Challenge, Advance and Emerging Opportunities for Metal-Organic Framework Glasses: from Dynamic Chemistry to Material Science and Noncrystalline Physics
Received date: 2022-12-23
Online published: 2023-02-16
Supported by
National Natural Science Foundation of China(22171075); BaGui Talent Program of Guangxi Province(2019AC26001); Young Teachers Grants from the Fok Ying-Tong Education Foundation(171110); Science and Technology Commission of Shanghai Municipality(22QC1401500); Science and Technology Commission of Shanghai Municipality(21DZ2260400)
The emerging metal-organic framework (MOF) glass, that is brand-new comer to the traditional glass and noncrystalline physics world, was viewed as the Holy Grail of future porous chemistry and the key direction of MOF derived functional materials. The known examples of MOF glass are extremely scarce, prepared mainly through the traditional melt-quenching method. As porous framework constructed from metal ions/clusters and organic linkers through coordinative bonds, the majority of MOFs can not reach high-temperature melt state, which prevents MOF glass formation. Facing these challenges, here we summarized the development history and latest advance of MOF glass. A new strategy of sequential perturbation based on dynamic chemistry was presented to widely prepare MOF glass. How to discover more MOF glasses, expand their properties and functions, and clarify their nature, is the new interdisciplinary frontier from dynamic chemistry to material science and noncrystalline physics. This topic also provides a range of new research opportunities, including the design and regulation of MOF glass based on reticular and dynamic chemistry, exploring new functions of MOF glass beyond its crystalline counterpart, and effectively responding to the scientific challenges in noncrystalline physics including the glass nature, based on the solid-solid structure transformation and relevance between crystalline and glassy MOFs.
Zheng Yin , Yingbo Zhao , Minghua Zeng . Challenge, Advance and Emerging Opportunities for Metal-Organic Framework Glasses: from Dynamic Chemistry to Material Science and Noncrystalline Physics[J]. Acta Chimica Sinica, 2023 , 81(3) : 246 -252 . DOI: 10.6023/A22120508
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