Advances in Electrochemical Reductive Removal of Oxyanions in Water★
Received date: 2023-04-13
Online published: 2023-06-12
Supported by
National Natural Science Foundation of China(22102100); National Natural Science Foundation of China(21936003); Natural Science Foundation of Shanghai(22ZR1431700); National Key Research and Development Program of China(2021YFA1201701); National Key Research and Development Program of China(2018YFC1800801)
The excessive discharge of oxyanions (i.e., nitrate, bromate, perchlorate) into water has caused more and more serious environmental pollution problems. Oxyanions are generally persistent, refractory, teratogenic and carcinogenic, posing a great threat to ecosystems and human health. Therefore, they have increasingly attracted widespread attention. Electrochemical reduction is regarded as one of the most promising water treatment technology, because it could employ either electrons or strong reductive species (atomic H*) generated by dissociating water molecules to realize the efficient, green and safe removal of toxic oxyanions. Herein, the electrochemical reduction mechanism for removing pollutants is briefly introduced, the advancements of electrochemical reduction of nitrate, bromate and perchlorate are summarized and their possible reaction pathways are discussed, the effect of catalysts (i.e., structure, types) on the performance of electrochemical reduction is further analyzed. Finally, the possible challenges of electrochemical reduction technology to remove oxyanions are deeply discussed and prospected.
Wei Hou , Yancai Yao , Lizhi Zhang . Advances in Electrochemical Reductive Removal of Oxyanions in Water★[J]. Acta Chimica Sinica, 2023 , 81(8) : 979 -989 . DOI: 10.6023/A23040133
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