煤矸石改性方法及其资源环境利用研究进展

doi:10.6023/A24010038

综述

煤矸石改性方法及其资源环境利用研究进展

张华林^a,b,c, 赵梦飞^a,b,c, 江晓亮^b, 田少静^b, 滕泽栋^a,e, 李庭刚^a,b,c,d,e,*

^a中国科学院过程工程研究所中国科学院绿色过程与工程重点实验室,中国科学院绿色过程制造创新研究院战略金属资源绿色循环利用国家工程研究中心北京市过程污染控制工程技术研究中心北京 100190;
^b中国科学院赣江创新研究院中国科学院稀土重点实验室江西省稀土清洁生产重点实验室赣州 341003;
^c江西理工大学冶金工程学院赣州 341099;
^d生物药制备与递送重点实验室(中国科学院) 生化工程国家重点实验室北京 100190;
^e中国科学院大学北京 100049

投稿日期:2024-01-29
作者简介:张华林,2022年江西理工大学与中国科学院赣江创新研究院联合培养在读博士研究生,主要从事方向为生态修复与改良.
赵梦飞,2021年江西理工大学与中国科学院赣江创新研究院联合培养在读博士研究生,主要从事方向为稀土生物浸出.
江晓亮,中国科学院赣江创新研究院助理研究员,主要从事矿山土壤改良、土壤重金属生态修复、重金属超富集植物与根际微生物互作机制研究.
田少静,2022年中国科学院赣江创新研究院在读博士研究生,主要从事环境功能材料设计与研发及其应用于稀土矿区的生态修复.
滕泽栋,中国科学院过程工程研究所副研究员,主要从事污染生态环境跨介质修复、环境生物技术强化减污降碳、环境功能材料设计与开发等方面的基础和应用研究.
李庭刚,博士,中国科学院过程工程研究所/中国科学院赣江创新研究院研究员,博士生导师,中国科学院过程所“百人计划”、江西省“千人计划”入选者.2008年获中国科学院生态环境研究中心博士学位,2006-2008年在新加坡南洋理工大学进行博士联合培养,2010-2019年在新加坡国立大学做博士后、特聘研究员,2019年至今在中国科学院过程工程研究所工作,环境生物技术课题组组长.中国科学院赣江创新研究院双聘.长期从事环境生物过程转化机理与能源资源化技术研究,主要涉及土壤-地下水修复、高盐有机废水处理与资源化、稀土生物冶金、生物新能源制造、环境污染物定向生物转化与功能材料应用基础研究.主持国家自然科学基金、国家重点研发计划项目课题、地方科技重大专项以及企业委托等科研项目.近年来在Science子刊Science Advances, Biotechnology for Biofuels, Environmental Science & Technology, Biotechnology and Bioengineering, Water Research, Bioresource Technology, Journal of Biotechnology, Renewable Energy等主流期刊上发表论文40余篇,申请和授权发明专利20余项.担任巴塞尔公约亚太区中心化学品和废物环境管理智库专家,中国自然资源学会废弃物资源化专业委员会委员,Clean Energy Science and Technology等期刊编委,Membrane期刊客座编辑,荣获2021年中国产学研促进会科技合作创新奖,2022年中国发明协会发明创业成果奖二等奖.
基金资助:
项目受鄂尔多斯市科技重大专项(2022EEDSKJZDZX014-1, 2022EEDSKJZDZX014-2)、江西省技术创新引导类计划项目(20212BDH81029)、稀土产业基金(IAGM2020DB06)、中国科学院重点部署项目(ZDRW-CN-2021-3-3)

Research Progress of Coal Gangue Modification Method and its Resource and Environment Utilisation

Hualin Zhang^a,b,c, Mengfei Zhao^a,b,c, Xiaoliang Jiang^b, Shaojing Tian^b, Zedong Teng^a,e, Tinggang Li^a,b,c,d,e,*

^aCAS Key Laboratory of Green Process and Engineering, Innovation Academy for Green Manufacture, National Engineering Research Center of Green Recycling for Strategic Metal Resources, Beijing Engineering Research Centre of Process Pollution Control, Institute of Process Engineering, Chinese Academy of Sciences, Beijing, 100190, China;
^bKey Laboratory of Rare Earth, Jiangxi Province Key Laboratory of Cleaner Production of Rare Earths, Ganjiang Innovation Academy, Chinese Academy of Sciences, Ganzhou 341003, China;
^cSchool of Metallurgical engineering, Jiangxi University of Science and Technology, Ganzhou 341099, China;
^dState Key Laboratory of Biochemical Engineering, Key Laboratory of Biopharmaceutical Preparation and Delivery, Chinese Academy of Sciences, Beijing, 100190, China;
^eUniversity of Chinese Academy of Sciences, Beijing 100049, China

Received:2024-01-29
Contact: * E-mail: tgli@ipe.ac.cn
Supported by:
Science and Technology Major Program of Ordos City of China (2022EEDSKJZDZX014-1, 2022EEDSKJZDZX014-2)、Technological Innovation Guidance Program of Jiangxi Province (20212BDH81029)、Rare Earth Industry Fund (IAGM2020DB06)、 the Key Research Program of the Chinese Academy of Sciences (ZDRW-CN-2021-3-3)

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摘要/Abstract

煤矸石是一种煤炭开采和洗选过程中产生的典型工业废弃物,其大量的堆积造成了较大的环境问题。通过不同的改性方法对煤矸石进行改性,可以显著提升其在环境保护、资源回收方面的应用潜力。改性煤矸石在环境应用方面的研究涉及多个领域,这些应用不仅有助于减轻煤矸石对环境的压力,而且可以通过回收和再利用,为环境保护和经济发展提供新的动力,实现煤矸石综合利用的可持续发展。本综述从煤矸石的环境问题出发,强调了通过改性技术提升其环保潜力的重要性并详细分析了改性煤矸石在废水处理、土壤修复、建筑材料制备等方面的应用,并探讨了面临的挑战和未来发展方向,为煤矸石资源化利用奠定了基础。

关键词: 煤矸石, 改性方法, 环境应用, 资源化

Coal gangue, a byproduct of coal mining and processing, has long been regarded as solid waste. However, with the increasing severity of resource scarcity and environmental pollution issues, the efficient utilization and resource recovery of coal gangue have become urgent needs. This paper reviews the modification and resource utilization of coal gangue, focusing on its introduction, pretreatment, modification methods, and the latest progress in resource utilization. Firstly, coal gangue is a porous granular material composed mainly of inorganic minerals, organic matter, and water. Due to its complex nature and diverse composition, the direct utilization of coal gangue is somewhat limited. Therefore, modifying coal gangue is a key step in achieving its resource utilization. Pretreatment before modification is a crucial step to ensure the effectiveness of coal gangue modification. This involves physical processes such as crushing, screening, magnetic separation, and washing of coal gangue to reduce particle size, achieve uniformity, enhance surface area and pore structure, thereby providing a solid foundation for subsequent modification. The modification methods of coal gangue mainly include chemical modification, biological modification, and composite modification. Chemical modification involves introducing functional groups or altering its chemical structure through processes such as acid-base treatment, organic modification, thermal activation, etc., thereby improving its adsorption performance, dispersibility, etc. Biological modification utilizes microorganisms, enzymes, and other biological systems to enhance the environmental friendliness and biocompatibility of coal gangue. Composite modification combines the advantages of various modifications to make coal gangue-based materials meet requirements better. Significant progress has been made in the resource utilization of coal gangue. Modified coal gangue is extensively utilized in environmental management sectors like soil remediation and wastewater treatment, showcasing excellent adsorption capabilities and catalytic activity. Furthermore, modified coal gangue is utilized as raw material in sectors such as construction materials, energy recovery, and fertilizer production, providing a new pathway for reducing mineral resource consumption and advancing circular economy development.

Key words: Coal gangue, Modification method, Environmental application, Resource recovery

引用此文

张华林, 赵梦飞, 江晓亮, 田少静, 滕泽栋, 李庭刚. 煤矸石改性方法及其资源环境利用研究进展[J]. 化学学报, doi: 10.6023/A24010038.

Hualin Zhang, Mengfei Zhao, Xiaoliang Jiang, Shaojing Tian, Zedong Teng, Tinggang Li. Research Progress of Coal Gangue Modification Method and its Resource and Environment Utilisation[J]. Acta Chimica Sinica, doi: 10.6023/A24010038.

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