共形二维材料: 创制与应用
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刘卫涛, 河南大学物理与电子学院在读博士生. 2018年毕业于郑州航空工业管理学院应用物理学专业, 同年进入河南大学物理与电子学院攻读硕士学位并于2020年转入硕博连读, 师从陈珂教授和黄明举教授. 研究方向为二维材料的生长调控与应用. |
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高战胜, 博士, 2023年毕业于南开大学材料学院, 同年入职河南大学物理与电子学院, 主要研究方向为低维材料及其异质结合成与器件表征. |
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黄明举, 博士, 河南大学教授. 河南省物理学会理事, 中国光学学会光学材料专业委员会委员, 国家高等学校“光电信息工程”类专业教学指导委员会协作分会委员, Opt. Eng.、Chin. Phys. Lett.、中国激光、光子学报等专业期刊审稿人. 河南省教育厅学术带头人, 省高校优秀骨干教师. 先后主持和参加国家自然科学基金等省部级以上项目11项, 获省部级以上优秀奖4项. 共发表SCI、EI论文160余篇. |
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刘忠范, 物理化学家, 日本东京大学博士. 北京大学博士生导师、博雅讲席教授、纳米科学与技术研究中心主任, 北京石墨烯研究院院长. 中国科学院院士、发展中国家科学院院士. 英国物理学会会士、英国皇家化学会会士、中国微米纳米技术学会会士. “物理化学学报”主编、“科学通报”副主编. 主要从事石墨烯等纳米碳材料研究, 在石墨烯、碳纳米管的化学气相沉积生长方法研究领域做出了一系列开拓性和引领性的工作. 发表SCI检索学术论文550余篇, 申请中国发明专利80余项. 曾获日中科技交流协会“有山兼孝纪念研究奖”(1992)、香港求是科技基金会杰出青年学者奖(1997)、中国分析测试协会科学技术奖一等奖(2005)、教育部高等学校科学技术奖自然科学一等奖(2007)、国家自然科学二等奖(2008)、中国化学会-阿克苏诺贝尔化学奖(2012)、宝钢优秀教师特等奖(2012)、日本化学会胶体与界面化学年会Lectureship Award(2016)、北京大学方正教师特别奖(2016)、“北京市优秀教师”称号(2017)、国家自然科学二等奖(2017)、ACS Nano Lectureship Award(2018)等. |
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陈珂, 河南大学教授, 博导, 国家万人计划青年拔尖人才(2020). 2012年获同济大学材料物理与化学博士学位并于同年入职河南大学. 2012年在英国剑桥大学化学系做访问博士生. 2013~2018年在北京大学化学与分子工程学院做博士后和访问学者. 2020~2021年在美国麻省理工学院材料科学与工程系做访问学者. 研究方向为二维材料的可控生长与纳米光学. 在Nat. Photon.、Nat. Commun.、Adv. Mater.等国际著名期刊共发表SCI论文60余篇, 参与编写石墨烯相关专著(章节)2部, 授权国家发明专利8项. 获河南省中原基础研究领军人才、中原青年拔尖人才、省教育厅学术技术带头人、省优秀青年专家、河南省青年科技奖等称号或奖励. |
收稿日期: 2024-07-17
网络出版日期: 2024-10-09
基金资助
国家自然科学基金(52272038); 国家自然科学基金(22309042); 国家万人计划和河南省中原英才计划的资助
Conformal Two-Dimensional Materials: Preparation and Applications
Received date: 2024-07-17
Online published: 2024-10-09
Supported by
National Natural Science Foundation of China(52272038); National Natural Science Foundation of China(22309042); National Young Top-Notch Talents of Ten-Thousand Talents Program and the Zhongyuan Talents Program of Henan Province
共形二维材料是指能与任意基底的表面形状“紧密贴合”的原子薄层材料, 它像薄膜一样紧密包覆于基底表面, 与基底表面轮廓融为一体, 进而形成一种新型的功能复合结构材料. 这种共形结构材料不仅继承了基底原始的表面形貌特征, 而且能将二维材料的新奇物性赋予基底材料而实现新的功能, 激发二维材料与基底相互作用下新的物理化学效应. 基底特殊结构的引入能够使二维材料超越二维空间的局限性, 将二维材料的平面结构与基底的任意曲面结构相结合, 是增强二维材料与外界物质相互作用的重要方式, 极大地拓展了二维材料的应用场景, 甚至可能实现其“杀手锏”应用. 本综述在提出共形二维材料概念的基础上, 阐明了二维材料共形生长的机制, 揭示了基底属性、结构对二维材料共形生长与共形度的影响规律, 探究了影响材料生长行为的热动力学因素与空间相平衡条件, 并分类综述了以基底的开放式结构和限域式结构为典型代表的共形二维材料的制备方法、性能与应用, 最后对该领域的挑战和未来发展方向做了展望.
刘卫涛 , 高战胜 , 黄明举 , 刘忠范 , 陈珂 . 共形二维材料: 创制与应用[J]. 化学学报, 2024 , 82(11) : 1162 -1179 . DOI: 10.6023/A24070219
Conformal two-dimensional materials refer to an atomically-thin layered material that can closely adhere on the surface of any substrate. It is tightly coated on the substrate surface like a thin film, along with the contour of the substrate surface, and thus forms a new type of functional composite structural material. This conformal structural material not only inherits the original surface morphological characteristics of the substrate, but also endows the substrate with novel physical properties of two-dimensional materials to achieve new functions and stimulate new physical and chemical effects under the interaction between two-dimensional materials and the substrate. The introduction of special substrate structures can enable two-dimensional materials to transcend the limitations of two-dimensional space. Combining the planar structure of two-dimensional materials with the arbitrary curved structure of the substrate is an important way to enhance interactions between two-dimensional materials and the surrounding environment, greatly expanding the application fields of two-dimensional materials, and may even achieve the killer applications. On the basis of proposing the concept of conformal two-dimensional materials, this article first elucidates the mechanism of conformal growth of two-dimensional materials, reveals the influence of substrate features and structures on the conformal growth and conformity of two-dimensional materials, as well as explores the thermodynamic factors and spatial equilibrium conditions that affect material growth behaviors. Second, it classifies and summarizes current progress on the preparation methods, properties, and applications of conformal two-dimensional materials represented by open and confined structures of substrates. Finally, the challenges and future development directions in this field are discussed.
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