Research Progress and Challenge of Aqueous Zinc Ion Battery

doi:10.6023/A20090409

Acta Chimica Sinica ›› 2021, Vol. 79 ›› Issue (2): 158-175.DOI: 10.6023/A20090409 Previous Articles Next Articles

Review

水系锌离子电池研究进展和挑战

张璐^a^,^b, 王文凤^a, 张洪明^a, 韩树民^a^,^b^,^*(), 王利民^a^,^b^,^*()

a 燕山大学环境与化学工程学院秦皇岛 066004
b 燕山大学亚稳材料制备技术与科学国家重点实验室秦皇岛 066004

投稿日期:2020-09-04 发布日期:2020-11-19
通讯作者: 韩树民, 王利民

作者简介:

张璐, 工学博士, 副教授. 2017年毕业于燕山大学, 曾获得2017年博士后创新人才支持计划, 2018年在美国俄勒冈州立大学从事博士后研究工作, 目前发表文章50余篇, 获授权专利11项, 河北省自然科学奖二等奖1项. 主要研究方向为新型电化学储能体系及器件和储氢材料.

王文凤, 博士研究生. 2016年起于燕山大学环境与化学工程学院攻读硕士学位, 2018年获得硕博连读资格, 攻读博士学位. 主要研究方向为储氢材料以及水系电池.

张洪明, 博士研究生. 2015年起于燕山大学环境与化学工程学院攻读硕士学位, 2017年获得硕博连读资格, 攻读博士学位. 主要研究方向为过渡金属催化剂作用下硼氢化合物水解制氢性能的研究.

韩树民, 博士生导师, 教授. 先后承担并主持完成或承担国家863计划和自然科学基金项目6项、省部级课题7项; 获授权国家发明专利20项, 发表SCI学术论文180篇, 获河北省技术发明奖二等奖2项; 担任Journal of Alloys and Compounds等杂志审稿人, 兼任国际电化学学会会员, 中国电化学委员会委员, 中国材料研究会产业工作委员. 近期的研究工作主要集中在新型稀土功能材料、新型电化学储能系统和器件的研究.

王利民, 博士生导师, 教授. 2019年入选教育部长江学者特聘教授、新世纪优秀人才支持计划等, 主持国家重点研发计划课题1项、国家自然科学基金5项、中国-意大利国际合作项目2项、科技部国家重点实验室基础研究项目8项、其他省部级项目10余项. 现任《Frontiers in Materials: glass science》副主编. 在Nature, Phys. Rev. Lett., Adv. Mater., J. Phys. Chem. Lett., Acta Mater.等SCI刊物上发表论文169篇, SCI他引超过4000次. 主要研究方向为非晶转变以及玻璃形变过程中的热力学和动力学研究.

* E-mail: hanshm@ysu.edu.cn;

* E-mail: limin_wang@ysu.edu.cn

基金资助:
国家自然科学基金(51701175); 国家自然科学基金(51971197); 河北省自然科学基金(E2020203081); 河北省自然科学基金(E2019203161)

Research Progress and Challenge of Aqueous Zinc Ion Battery

Lu Zhang^a^,^b, Wenfeng Wang^a, Hongming Zhang^a, Shumin Han^a^,^b^,^*(), Limin Wang^a^,^b^,^*()

a School of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao 066004, China
b State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004, China

Received:2020-09-04 Published:2020-11-19
Contact: Shumin Han, Limin Wang
Supported by:
National Natural Science Foundation of China(51701175); National Natural Science Foundation of China(51971197); Natural Science Foundation of Hebei Province(E2020203081); Natural Science Foundation of Hebei Province(E2019203161)

Aqueous zinc ion batteries (AZIBs) as an emerging battery energy storage technology have attracted widespread attention and developed rapidly in recent years due to the merits of high safety, low price, high energy density, environmental friendliness, easy manufacturing, etc., showing good application value and prospect in large-scale energy storage and other fields. Embarking from the current scientific issues existed in AZIBs, we review the important progress in cathode and anode materials and electrolyte used in AZIBs in this article. Firstly, the characteristics of multiple cathode materials that developed and their electrochemical reaction mechanism are analyzed and summarized. Afterward, the challenge and improving strategy for metal zinc anode are discussed, and the features of different aqueous electrolytes and the optimization solution are analyzed. Finally, the scientific problems to solve and technical challenges for the practical application in the future of this novel battery technology are summarized and prospected.

Key words: aqueous zinc ion battery, zinc anode, cathode material, electrolyte, energy storage

Cite this article

Lu Zhang, Wenfeng Wang, Hongming Zhang, Shumin Han, Limin Wang. Research Progress and Challenge of Aqueous Zinc Ion Battery[J]. Acta Chimica Sinica, 2021, 79(2): 158-175.

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Fig. & Tab. 8

Figure 1. Mechanism of aqueous zinc ion batteries

Figure 2. (a) The crystal structure of MnO2. (b) Schematic illustration of the pre-intercalated Na+-MnO2 to increase structural stability and ion diffusion[18] (Copyright 2019, American Chemical Society). (c) Schematic illustration of the preparation of polyaniline (PANI)-intercalated MnO2 [19] (Copyright 2018, Springer Nature)

Figure 3. (a) Schematic illustration of mechanism of Zn||α-MnO2 cell in 3 mol/L Zn(CF3SO3)2+0.1 mol/L Mn(CF3SO3)2 electrolyte[24] (Copyright 2017, Springer Nature). The XRD patterns (b) after fully charged and (c) discharged to 1 V and charged back to 1.8 V of α-MnO 2, and (d) STEM-EDS mappings of α-MnO 2discharged to 1 V[20] (Copyright 2016, Springer Nature). (e) Discharge galvanostatic intermittent titration technique (GITT) proﬁles of the Zn||α-MnO2 cell with the morphology of α-MnO 2 inserted[28] (Copyright 2017, American Chemical Society). (f) Galvanostatic charge/discharge (GCD) profiles within 100 cycles and (g) schematic illustration of electrochemical mechanism of ε-MnO 2 in 1 mol/L ZnSO4+1 mol/L MnSO4 electrolyte[31] (Copyright 2019, Wiley-VCH)

Figure 4. (a) Crystal structure of layered V2O5. (b) Schematic illustration mechanism, (c) GCD profiles at a 1C (300 mA/g), and (d) discharge profiles at 4C to 20C rates of Zn0.25V2O5•nH2O cathode[38] (Copyright 2016, Springer Nature). (e) Cycling performance of VOG (V2O5•nH2O/graphene) and VOG-350 (annealing VOG at 350 ℃ for 2 h) at 6 A/g[39] (Copyright 2018, Wiley-VCH). (f) Schematic illustration of the energy versus DOS and (g) GCD profiles comparison of Co0.247V2O5•0.944H2O and V2O5•nH2O cathodes[40] (Copyright 2019, Wiley-VCH)

Figure 5. (a) Crystal structure of the metal hexacyanoferrates (MHCFs). (b) Rate discharge curves of Zn3[Fe(CN)6]]2 (ZnHCF) in 1 mol/L ZnSO4 electrolyte[64] (Copyright 2015, Wiley-VCH). (c) Schematic illustration of reversible Zn2+ intercalation/deintercalation during electrochemical process of CoFe(CN)6, (d) GCD profiles at different current densities of CoFe(CN)6, and (e) comparison of capacity versus voltage with reported MHCFs cathodes for AZIBs of CoFe(CN)6 [66] (Copyright 2019, Wiley-VCH)

Figure 6. (a) Discharge/charge voltages and capacities of selected quinone compounds in 3 mol/kg Zn(CF3SO3)2 electrolyte, compared with some reported cathodes. (b) Galvanostatic discharge/charge curves of C4Q/Zn battery at the current density of 20 mA/g[74] (Copyright 2018, American Association for the Advancement of Science). (c) Cyclic voltammograms (CV) of the Zn anode against the p-chloranil cathode in 1 mol/L Zn(CF3SO3)2 electrolyte. (d) Structural change models of p-chloranil upon Zn2+ insertion[75] (Copyright 2018, American Chemical Society). (e) Structural formula and (f) comparison of GCD files of PQ-△ using 0.25 mol/L Zn(CF3SO3)2 organic (MeCN solvent) and 3 mol/L Zn(CF3SO3)2 aqueous electrolytes of PQ-△[76] (Copyright 2020, American Chemical Society). (g) Long-term cycling performance of Zn||DTT battery[78] (Copyright 2018, Wiley-VCH)

Figure 7. (a) Schematic diagram of the issues for Zn anodes in aqueous electrolytes. (b) Schematic illustrations of Zn deposition on CC and CNT electrodes[88] (Copyright 2019, Wiley-VCH). (c) Schematic illustration of the Zn plating on ZIF-8, and (d) SEM images of Zn deposits at a current density of 1.0 mA/cm2 for different capacities on ZIF-8[89] (Copyright 2019, Elsevier). (e) Scheme illustrating the design principle of epitaxial zinc metal electrodeposition[92] (Copyright 2019, American Association for the Advancement of Science). Schematic diagrams for Zn deposition on a bare (f) and the PA layer coating (g) electrodes, and (h) long-term galvanostatic cycling of symmetrical Zn cells[96](Copyright 2019, Elsevier). (i) In situ optical microscope images of the front surfaces of Zn and PVB@Zn electrodes[99] (Copyright 2020, Wiley-VCH). (j) Schematic illustration of desolvation process of Zn2+-H2O ion on bare Zn and coating anodes[103] (Copyright 2020, Wiley-VCH). (k) SEM image and XRD pattern (inset) of a Zn anode after 500 stripping/plating cycles in 1 mol/kg Zn(TFSI)2+20 mol/kg LiTFSI electrolyte[104] (Copyright 2018, Springer Nature). CEs of Zn plating/stripping in asymmetric Zn/Zn cells in (l) 5 mol/kg and (m) 30 mol/kg ZnCl2 electrolytes[105] (Copyright 2018, Royal Society of Chemistry). (n) Impact of organic additives in electrolyte on cyclability of zinc anode[108] (Copyright 2017, American Chemical Society)

Figure 8. CV of Zn electrode in (a) 1 mol/L ZnSO4 and (b) 1 mol/L Zn(CF3SO3)2 aqueous electrolyte[114] (Copyright 2016, American Chemical Society). (c) Cycling stability of Ca0.20V2O5•0.80H2O cathode in different concentrated ZnCl2 electrolytes[45] (Copyright 2019, Wiley-VCH). (d) The cycling stability of the Na3V2(PO4)2O2F electrode in the 25 mol/kg ZnCl2+5 mol/kg NH4Cl and 30 mol/kg ZnCl2 electrolytes[121] (Copyright 2020, Wiley-VCH). (e) CV curves of Zn electrodes and (f) second GCD curves of Zn/VOPO4 batteries in different electrolytes[72] (Copyright 2019, Wiley-VCH). (g) Radar chart comparison of common used conventional and concentrated aqueous electrolytes. (h) Radar chart comparison of the performance of common used conventional and concentrated aqueous electrolytes with desired aqueous electrolyte. (i) The usage of electrolytes of AZIBs

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水系锌离子电池研究进展和挑战

Research Progress and Challenge of Aqueous Zinc Ion Battery

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