Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides
Received date: 2019-07-11
Online published: 2019-09-05
Supported by
the National Natural Science Foundation of China(21871021);the National Natural Science Foundation of China(21521005);the National Key Research and Development Program(2017YFA0206804);the Fundamental Research Funds for the Central Universities(buctylkxj01);the Fundamental Research Funds for the Central Universities(XK1802-6)
Supported catalysts have been widely used in a large variety of industrial processes, including ammonia synthesis, energy conversion and fine chemical synthesis. Layered double hydroxides (LDHs) are a class of two-dimensional functional anionic materials. By virtue of the unique structural characteristics (e.g., tunability of host layers, high dispersion of metal cations and structure topological transformation), LDHs have shown potential applications in heterogeneous catalysis as precursors or supports. In this review, high-performance monometallic or bimetallic supported catalysts by using LDHs as supports/precursors, or by utilizing mixed metal oxides (MMO) as supports via topotactic transformation from LDHs is highlighted. Their recent progresses in electrocatalysis, oxidative dehydrogenation, selective hydrogenation and syngas conversion reaction are reviewed. In the final section, future opportunities and challenges in the preparation of LDHs-based catalysts are discussed, and some strategies to resolve these critical problems are further proposed.
Jun Yu , Yusen Yang , Min Wei . Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides[J]. Acta Chimica Sinica, 2019 , 77(11) : 1129 -1139 . DOI: 10.6023/A19070260
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