Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides

doi:10.6023/A19070260

Acta Chimica Sinica ›› 2019, Vol. 77 ›› Issue (11): 1129-1139.DOI: 10.6023/A19070260 Previous Articles Next Articles

Review

水滑石基负载型催化剂的制备及其在催化反应中的应用

余俊, 杨宇森*(), 卫敏*()

北京化工大学化学学院化工资源有效利用国家重点实验室北京 100029

投稿日期:2019-07-11 发布日期:2019-09-05
通讯作者: 杨宇森,卫敏 E-mail:2016400160@mail.buct.edu.cn;weimin@mail.buct.edu.cn
作者简介:余俊, 北京化工大学在读研究生, 2018年6月于北京化工大学理学院应用化学专业获得学士学位, 随后加入北京化工大学化工资源有效利用国家重点实验室卫敏教授课题组, 主要研究方向为超分子插层与自组装|杨宇森, 男, 博士, 1991年6月出生于浙江嘉兴, 2014年6月在北京化工大学理学院应用化学专业获得学士学位, 随后加入北京化工大学化工资源有效利用国家重点实验室卫敏教授课题组, 并于2019年6月获得化学工程与技术专业博士学位.博士阶段主要研究水滑石基负载型催化剂的制备及其对选择性加氢反应的催化性能|卫敏, 女, 教授, 博士生导师. 2001年于北京大学获理学博士学位. 2008年佐治亚理工学院访问学者. 2001年至今于北京化工大学从事插层化学与功能材料研究.研究方向: (1)插层结构功能材料的结构设计、组装与性能调控; (2)新型催化材料的结构设计和性能研究.近5年以通讯作者在J. Am. Chem. Soc.、Angew. Chem., Int. Ed.和Adv. Mater.等刊物发表SCI收录研究论文90余篇; 他引9700余次, 单篇最高他引430余次. 2016年入选英国皇家化学会会士; 现担任Science Bulletin期刊副主编, 催化学报编委.获2012年国家杰出青年基金资助.获2015年中国石油和化学工业联合会科技进步一等奖.入选2017年度科技部中青年科技创新领军人才和国家百千万人才工程, 被授予“有突出贡献中青年专家”称号.获2018年第十五届中国青年科技奖
基金资助:
国家自然科学基金(21871021);国家自然科学基金(21521005);国家重点研发计划(2017YFA0206804);中央高校基本科研业务费(buctylkxj01);中央高校基本科研业务费(XK1802-6)

Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides

Yu Jun, Yang Yusen*(), Wei Min*()

State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology, Beijing 100029

Received:2019-07-11 Published:2019-09-05
Contact: Yang Yusen,Wei Min E-mail:2016400160@mail.buct.edu.cn;weimin@mail.buct.edu.cn
Supported by:
the National Natural Science Foundation of China(21871021);the National Natural Science Foundation of China(21521005);the National Key Research and Development Program(2017YFA0206804);the Fundamental Research Funds for the Central Universities(buctylkxj01);the Fundamental Research Funds for the Central Universities(XK1802-6)

Supported catalysts have been widely used in a large variety of industrial processes, including ammonia synthesis, energy conversion and fine chemical synthesis. Layered double hydroxides (LDHs) are a class of two-dimensional functional anionic materials. By virtue of the unique structural characteristics (e.g., tunability of host layers, high dispersion of metal cations and structure topological transformation), LDHs have shown potential applications in heterogeneous catalysis as precursors or supports. In this review, high-performance monometallic or bimetallic supported catalysts by using LDHs as supports/precursors, or by utilizing mixed metal oxides (MMO) as supports via topotactic transformation from LDHs is highlighted. Their recent progresses in electrocatalysis, oxidative dehydrogenation, selective hydrogenation and syngas conversion reaction are reviewed. In the final section, future opportunities and challenges in the preparation of LDHs-based catalysts are discussed, and some strategies to resolve these critical problems are further proposed.

Key words: layered double hydroxides, topological transformation, preparation method, high dispersion, supported catalyst

Cite this article

Yu Jun, Yang Yusen, Wei Min. Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides[J]. Acta Chimica Sinica, 2019, 77(11): 1129-1139.

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Fig. & Tab. 10

Figure 1. Proposed mechanism of Pd loaded on MgAl-LDH(HT) and MgO supports[49]

Figure 2. Schematic illustration for the preparation of Au@TiO2－x/ZnO and Au@ZnO/TiO2[38]

Figure 3. Schematic illustration for the preparation of structured Cu@(CuCo-alloy)/Al2O3 catalyst with a core-shell architecture derived from the CuCoAl-LDH film[55]

Figure 4. (a) Schematic illustration for the hydrolysis-deposition to form Ru/CoFe-LDHs, (b) transmission electron microscopy (TEM) images of as-prepared Ru/CoFe-LDHs nanosheets (inset shows the corresponding SAED pattern of Ru/CoFe-LDHs nanosheets marked in orange circle), (c) Cs-corrected STEM image of Ru/CoFe-LDHs nanosheets shows the monoatomic ruthenium dispersed on the surface of LDHs (some of the isolated Ru atoms are marked with red circles) and (d) HAADF-STEM images of the Ru/CoFe-LDHs and corresponding elemental distribution maps of Ni, Fe, and Ru in the Ru/CoFe-LDHs[66]

Figure 5. Schematic illustration and HRTEM images of Au/MgAl-LDH with different loading prepared by homogeneous precipitation-deposition technique[32]

Figure 6. Schematic illustration for the oxidant-free dehydrogenation of 2-octanol over Ni/NiAl-MMO catalyst[85]

Figure 7. Conceptual model for the selective acetylene hydrogenation mechanism on PdAg/Mg0.5Ti0.5Oy catalysts[90]

Figure 8. Schematic illustration for the selective hydrogenation of cinnamaldehyde to cinnamol catalyzed by Co-Ga intermetallics[94]

Figure 9. Schematic illustration for selective hydrogenation of furfural in the presence of two types of Ni nanoparticles with different surface fine structure[8]

Figure 10. Schematic illustration for the preparation of CuCo-alloy/ Al2O3/CNTs composites and catalytic performance towards higher alcohols synthesis from syngas[102]

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水滑石基负载型催化剂的制备及其在催化反应中的应用

Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides

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