Catalytic Synthesis of Nitrogen-doped Bamboo-shaped Carbon Nanotubes

Acta Chimica Sinica ›› 2007, Vol. 65 ›› Issue (10): 913-916. Previous Articles Next Articles

Original Articles

氮掺杂竹节状碳纳米管的催化合成

王利军*^,1, 解丽丽¹, 李永伦², 袁昊¹, 李庆华¹, 李全芝³

(¹上海第二工业大学环境工程系环境功能材料实验室上海 201209)
(²神华煤制油研究中心有限公司科研管理部上海 201108)
(³复旦大学化学系分子催化与创新材料实验室上海 200433)

投稿日期:2006-08-24 修回日期:2006-11-27 发布日期:2007-05-28
通讯作者: 王利军

Catalytic Synthesis of Nitrogen-doped Bamboo-shaped Carbon Nanotubes

WANG Li-Jun*^,1; XIE Li-Li¹; LI Yong-Lun²; YUAN Hao¹; LI Qing-Hua¹; LI Quan-Zhi³

(¹Department of Environmental Engineering, Shanghai Second Polytechnic University, Shanghai 201209)
(²Department of Scientific Research Management, Shenhua Coal-to-Oil Research Center Ltd., Shanghai 201108)
(³Laboratory of Molecular Catalysis and Innovative Materials, Department of Chemistry, Fudan University, Shanghai 200433)

Received:2006-08-24 Revised:2006-11-27 Published:2007-05-28
Contact: WANG Li-Jun

Abstract

Bamboo-shaped, nitrogen-doped, large-inner diameter carbon nanotubes were synthesized by catalytic method with organic amine as carbon and nitrogen source. By Fe/SBA-15 molecular sieve catalyst, nitrogen-doped bamboo-shaped carbon nanotubes (CN_X) were synthesized at 973 K high cracking reaction temperature. The effects of Fe content, diethylamine and hexamethylene tetraamine source on the shape and nitrogen-doped content of CN_X were discussed. Nitrogen-doped bamboo-shaped carbon nanotubes with N/C ratio of 0.26 were synthesized.

Key words: organic amine, bamboo-shaped, nitrogen-doped, carbon nanotube, catalytic synthesis

Cite this article

WANG Li-Jun*^,1; XIE Li-Li; LI Yong-Lun²; YUAN Hao; LI Qing-Hua; LI Quan-Zhi³. Catalytic Synthesis of Nitrogen-doped Bamboo-shaped Carbon Nanotubes[J]. Acta Chimica Sinica, 2007, 65(10): 913-916.

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氮掺杂竹节状碳纳米管的催化合成

Catalytic Synthesis of Nitrogen-doped Bamboo-shaped Carbon Nanotubes

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