无机钙钛矿太阳能电池稳定性研究进展

doi:10.6023/A19110411

化学学报 ›› 2020, Vol. 78 ›› Issue (3): 217-231.DOI: 10.6023/A19110411 上一篇下一篇

综述

无机钙钛矿太阳能电池稳定性研究进展

杨英^a,b,c, 林飞宇^a,b,c, 朱从潭^a,b,c, 陈甜^a,b,c, 马书鹏^a,b,c, 罗媛^a,b,c, 朱刘^d, 郭学益^a,b,c

a 中南大学冶金与环境学院长沙 410083;
b 有色金属资源循环利用湖南省重点实验室长沙 410083;
c 有色金属资源循环利用湖南省工程研究中心长沙 410083;
d 广东先导稀材股份有限公司广东 511500

投稿日期:2019-11-22 发布日期:2020-01-13
通讯作者: 郭学益 E-mail:xyguo@csu.edu.cn
作者简介:杨英,副教授,武汉大学博士毕业.长期从事材料物理化学及新能源材料与器件的科研工作,对固态高分子电解质以及固态染料敏化太阳能电池、量子点太阳能电池及钙钛矿太阳能电池有夯实的理论和实践基础.于2013~2014年间美国怀俄明大学完成博士后研究工作.现工作于中南大学冶金与环境学院.主要研究方向:新能源材料与器件;郭学益,教授,1995年于中南大学获得博士学位.1997年完成博士后研究工作,1999~2000年在日本佐贺大学理工学部机能物质化学科担任研究员,2000~2003年在日本东京大学国际产学共同研究中心担任客员教授.现工作于中南大学冶金与环境学院.主要研究方向:资源循环利用及环境材料.
基金资助:
项目受国家自然科学基金（No.61774169）、留学回国基金资助以及中南大学研究生自主探索创新项目（No.2019zzts944，502211922）资助.

Research Progress in the Stability of Inorganic Perovskite Solar Cells

Yang Ying^a,b,c, Lin Feiyu^a,b,c, Zhu Congtan^a,b,c, Chen Tian^a,b,c, Ma Shupeng^a,b,c, Luo Yuan^a,b,c, Zhu Liu^d, Guo Xueyi^a,b,c

a School of Metallurgy and Environment, Central South University, Changsha 410083;
b Hunan Key Laboratory of Nonferrous Metal Resources Recycling, Changsha 410083;
c Hunan Engineering Research Center of Nonferrous Metal Resources Recycling, Changsha 410083;
d First Rare Materials Co., Ltd, Guangdong 511500

Received:2019-11-22 Published:2020-01-13
Supported by:
Project supported by the National Natural Science Foundation of China (No. 61774169), Scientific Research Foundation for the Returned overseas Chinese Scholar; Postgraduate Independent Exploration and Innovation Projects of Central South University (Nos. 2019zzts944, 502211922).

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摘要/Abstract

近年来钙钛矿太阳能电池发展迅速，全无机钙钛矿具有良好的热稳定性、高吸光系数、带隙可调、制备简单等优点备受关注.现今，无机钙钛矿太阳能电池的最高光电转化效率已达19.03%，具有很好的发展潜力.本综述将从无机钙钛矿太阳能电池的制备方法、薄膜掺杂、界面修饰对稳定性影响入手，系统介绍无机钙钛矿太阳能电池的发展并进行分析总结，并着重分析了无机钙钛矿不稳定的原因及其改善方法，最后对于无机钙钛矿太阳能电池的未来进行了展望.

关键词: 无机钙钛矿太阳能电池, 制备方法, 界面修饰, 薄膜掺杂, 稳定性提高

In recent years, the efficiency of perovskite solar cells has developed rapidly, but its stability is limited by the influence of heat, light and water. All-inorganic perovskite formed by inorganic cations instead of organic cations shows improved thermal stability, high light absorption and adjustable band gap. The photoelectric conversion efficiency of all-inorganic perovskite solar cells has been improved to 19.03% at present. Among them, CsPbI₃ perovskite solar cells have good photoelectric performance but poor stability, while CsPbBr₃ perovskite solar cells have excellent stability but poor photoelectric performance of devices. In this paper, the influence of preparation method, film doping and interface modification on the stability of inorganic perovskite solar cells is systematically summarized. The reasons behind the instability of inorganic perovskite and the improvement methods are emphatically analyzed. In conclusion, improving the stability of inorganic perovskite light absorbing materials by film doping, surface passivation and morphology control such as low dimensional materials preparation can effectively improve the stability of the overall device, which provides the basis for further commercialization. In addition, it is of great significance to study the theory of charge transfer and recombination and establish a complete theoretical system for improving the performance and stability of the device. At present, most of perovskite contains harmful elements Pb. How to replace Pb and find new materials applied in perovskite solar cells is also the future development trend. In a word, as a new type of solar cell, inorganic perovskite solar cell is expected to contribute to the photovoltaic development of the future society.

Key words: inorganic perovskite solar cell, preparation method, interface modification, film doping, improved stability

引用此文

杨英, 林飞宇, 朱从潭, 陈甜, 马书鹏, 罗媛, 朱刘, 郭学益. 无机钙钛矿太阳能电池稳定性研究进展[J]. 化学学报, 2020, 78(3): 217-231.

Yang Ying, Lin Feiyu, Zhu Congtan, Chen Tian, Ma Shupeng, Luo Yuan, Zhu Liu, Guo Xueyi. Research Progress in the Stability of Inorganic Perovskite Solar Cells[J]. Acta Chimica Sinica, 2020, 78(3): 217-231.

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无机钙钛矿太阳能电池稳定性研究进展

Research Progress in the Stability of Inorganic Perovskite Solar Cells

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