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王金凤, 湖北黄冈人, 博士研究生, 天津大学工程师, 2019年于武汉大学获得理学博士学位, 主要从事染料敏化太阳能电池、室温磷光和力致发光相关研究. |
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李振, 湖北孝感人, 教授, 国家杰出青年科学基金获得者, “科技部中青年科技创新领军人才计划”入选者, 国家“万人计划”入选者, 英国皇家化学会会士(Fellow of RSC). 1997年于武汉大学化学系获理学学士学位, 2002年于武汉大学化学学院获理学博士学位. 研究方向为有机、高分子光电功能材料化学. 研究对象主要为有机共轭体系和功能高分子, 研究范围涉及二阶非线性光学、有机室温磷光、力致发光、聚集诱导发光、传感器、太阳能电池、磁性纳米材料等. |
收稿日期: 2021-01-28
网络出版日期: 2021-03-19
基金资助
项目受天津大学启动基金资助
Significant Influence of Molecular Packing in Aggregates on Optoelectronic Properties
Received date: 2021-01-28
Online published: 2021-03-19
Supported by
Starting Foundation of Tianjin University
有机小分子材料是由许多分子构成的聚集体, 其性能既与单个分子的空间构型和电子特性有关, 更与聚集体中分子的排列方式和分子间相互作用密切相关. 在有机小分子材料中, 聚集体的性质并不是组成它的单分子行为的简单线性叠加, 而是经常呈现出聚集态的整体差异性响应特点, 即: 不同的聚集态分子排列引起截然不同的性能. 因此, 科学研究已逐渐由单分子研究迈向分子聚集态科学. 随着人们对分子聚集态科学的关注, 特别是对有机分子固态下的排列和堆积方式、分子间相互作用等方面的深入研究发现, 通过不同策略对分子聚集态行为的有效调控, 可以实现完全不同于单个分子特性的聚集态发光现象, 包括发光强度、颜色、形式以及激发过程的差异. 也可以通过分子聚集态的形貌和维度的调节, 实现不同光电器件性能的调节和优化. 本综述将分别介绍聚集态分子的排列方式对力致变色、室温磷光、力致发光和有机场效应晶体管等方面的重要影响, 进一步阐述聚集态分子行为的重要性, 同时, 为有效调控聚集态分子的排列方式, 有针对性地设计和开发优异性能的光电材料提供基础.
王金凤 , 李振 . 聚集态分子排列对光电性能的影响[J]. 化学学报, 2021 , 79(5) : 575 -587 . DOI: 10.6023/A21010029
Organic materials based on small molecules are aggregates that composed of many molecules. Their properties are not only determined by the spatial configuration and electronic properties of individual molecule, but also closely related to the molecular packing modes and the intermolecular interactions in the aggregates. In the realm of organic molecules, the macroscopic performance of molecular aggregates is not just the simple superposition of single molecules, but often display overall differential response of aggregates, namely, distinct properties can be created by molecular uniting with particular packing modes. Therefore, molecular aggregation science has gradually appeared in scientific research and drawn much attention in recent years. With the continuous and serious exploration of molecular aggregation science, especially the in-depth study of the molecular packing modes and intermolecular interactions of organic molecules in the solid state, it is found that the luminescence based on aggregation state is completely different from the characteristics of individual molecule, including the emission intensity and color, emission type, and even the excitation process, which could be realized by regulating molecular aggregation behavior. In addition, the morphology and dimensions of the aggregates can also be adjusted to achieve excellent performances of optoelectronic devices. This review will introduce the important influence of the arrangement of aggregated molecules on mechanochromism, room temperature phosphorescence, mechanoluminescence and organic field effect transistors, and further elaborate the importance of the molecular packing, providing some guidance for regulating molecular packing mode and targeted design and development of high-performance optoelectronic materials.
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〉 |
