第二代生物柴油制备的多相催化剂的结构设计及研究进展
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田钊炜, 女, 北京化工大学在读研究生, 2021年6月于北京化工大学材料科学与工程学院材料科学与工程专业, 获得学士学位, 随后加入北京化工大学化工资源有效利用国家重点实验室卫敏教授课题组, 主要研究方向为第二代生物柴油的制备和发展. |
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杨宇森, 博士, 副教授, 硕士生导师. 2019年于北京化工大学获得化学工程与技术博士学位, 师从卫敏教授. 2019年至今在北京化工大学化工资源有效利用国家重点实验室从事多相催化研究, 主要研究方向: (1)生物质平台分子的定向催化转化; (2)可再生资源途径制氢、氢气精制与高效利用. 目前, 已发表SCI研究论文40余篇. 以第一(含共一)作者和共同通讯作者在Nat. Commun.、ACS Catal.、Appl. Catal. B: Environ.、J. Catal.、Green Chem.、《化学学报》及《化工学报》等期刊发表学术论文25篇(其中IF>10的16篇), 申请国家发明专利6件(其中获得授权1件). |
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卫敏, 女, 教授, 博士生导师. 2001年于北京大学获理学博士学位. 2008年佐治亚理工学院访问学者. 2001年至今于北京化工大学从事插层化学与功能材料研究. 研究方向: (1)插层结构功能材料的结构设计、组装与性能调控; (2)新型催化材料的结构设计和性能研究. 近5年以通讯作者在J. Am. Chem. Soc.、Angew. Chem., Int. Ed.、Nat. Commun.等刊物发表SCI收录研究论文90余篇; 他引11700余次. 2016年入选英国皇家化学会会士; 现担任Sci. Bull.期刊副主编, 催化学报编委. 获2012年国家杰出青年基金资助. 获2015年中国石油和化学工业联合会科技进步一等奖. 入选2017年度科技部中青年科技创新领军人才和国家百千万人才工程, 被授予“有突出贡献中青年专家”称号. 获2018年第十五届中国青年科技奖. |
收稿日期: 2022-04-26
网络出版日期: 2022-07-04
基金资助
北京自然科学基金(2212012); 国家自然科学基金(22172006); 国家自然科学基金(21521005); 国家自然科学基金(22102006); 国家重点研发计划(2021YFC2103501); 中央高校基本科研业务费(XK1803-05)
Structural Design and Research Progress of Heterogeneous Catalysts for the Preparation of Second Generation Biodiesel
Received date: 2022-04-26
Online published: 2022-07-04
Supported by
Beijing Natural Science Foundation(2212012); National Natural Science Foundation of China(22172006); National Natural Science Foundation of China(21521005); National Natural Science Foundation of China(22102006); National Key Research and Development Program(2021YFC2103501); Fundamental Research Funds for the Central Universities(XK1803-05)
生物柴油是一种重要的可再生清洁能源, 特别是经催化加氢脱氧等系列过程制备的第二代生物柴油, 在成分上与石油基燃料相似, 有望成为一种替代传统化石燃料的绿色能源. 在合成第二代生物柴油的研究中, 设计与制备兼具高活性与高稳定性的加氢脱氧多相催化剂是关键问题. 近年来, 研究者对于催化剂的种类与应用进行了探索, 并取得了一定的进展. 详细分析了加氢脱氧制备第二代生物柴油反应原料及反应参数、反应器对生产路径和产能的影响, 并对反应机理进行了介绍; 进一步从双金属位点、金属-酸性位点及金属-空位协同作用三个方面对催化剂结构设计进行了讨论和分析; 最后, 对第二代生物柴油领域的未来发展趋势进行了展望.
田钊炜 , 达伟民 , 王雷 , 杨宇森 , 卫敏 . 第二代生物柴油制备的多相催化剂的结构设计及研究进展[J]. 化学学报, 2022 , 80(9) : 1322 -1337 . DOI: 10.6023/A22040189
Biodiesel is an important renewable and clean energy, especially the second-generation of biodiesel prepared by a series of processes such as catalytic hydrodeoxygenation. It is similar to petroleum-based fuels in composition, and is expected to become a green energy alternative to traditional fossil fuels. In the study of the synthesis of the second generation of biodiesel, the design and preparation of hydrodeoxygenation heterogeneous catalysts with high activity and stability are the key issues. In recent years, many studies have been reported on the types and applications of catalysts, and some research progress has been made. The effects of reaction materials, reaction parameters and reactor on the production path and capacity of the second generation biodiesel prepared by hydrodeoxygenation were surveyed in detail, and the reaction mechanism was introduced. Then regulation strategies of hydrodeoxygenation catalysts are discussed and analyzed from three aspects: bimetallic sites, metal-acidic sites and metal-vacancy synergistic effect. In the final section, future development opportunities and challenges for the second-generation biodiesel are prospected.
Key words： biomass; biodiesel; hydrodeoxygenation; heterogeneous catalyst; synergistic effect
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