Recent Advances and Application Prospects in Photothermal Materials★

doi:10.6023/A23050232

Acta Chimica Sinica ›› 2023, Vol. 81 ›› Issue (10): 1420-1437.DOI: 10.6023/A23050232 Previous Articles Next Articles

Special Issue: 庆祝《化学学报》创刊90周年合辑

Review

光热材料的发展现状及应用前景^★

徐赫^a^,^b, 韩鹏博^a^,^b, 秦安军^a^,^b^,^*(), 唐本忠^b^,^c^,^d

a 华南理工大学发光材料与器件国家重点实验室广东省分子聚集发光重点实验室广州 510640
b 华南理工大学聚集诱导发光研究中心广州 510640
c 香港中文大学(深圳)理工学院深圳分子聚集体科学与工程研究院深圳 518172
d 香港科技大学国家人体组织功能重建工程技术研究中心香港分中心香港 999077

投稿日期:2023-05-17 发布日期:2023-07-13

作者简介:

徐赫, 2021年在合肥工业大学获得学士学位, 现为华南理工大学2021级硕士研究生. 研究兴趣是有机/聚合物光热功能材料.

秦安军, 1999 年和2004 年分别在山西大学和中国科学院化学研究所获得学士和博士学位. 2005至2008年先后在香港科技大学化学系和浙江大学高分子科学与工程学系从事博士后研究. 2008 年12月起先后任浙江大学副研究员、副教授, 2013年9月至今任华南理工大学教授、博导. 研究兴趣为高分子合成化学以及有机/聚合物功能材料. 曾获国家自然科学一等奖(2017, 2/5). 目前, 担任Aggregate《聚集体》期刊责任主编.

唐本忠, 1982年和1988年分别在华南理工大学和日本京都大学获得学士学位和博士学位, 于1989~1994年在加拿大多伦多大学从事博士后研究. 1994年加盟香港科技大学, 2009年、2017年、2020年先后当选中国科学院院士、亚太材料科学院院士、发展中国家科学院院士. 2021年加入香港中文大学(深圳)并担任理工学院院长、校长学勤讲座教授. 主要从事高分子化学和先进功能材料研究, 是AIE概念的提出者和AIE研究的引领者. 2014年至今连续入选ESI材料和化学双领域“高被引科学家”. 曾获Biomaterials Global Impact Award, Nano Today国际科学奖、2017年度国家自然科学一等奖、何梁何利基金科学与技术进步奖等奖项.

^★庆祝《化学学报》创刊90周年.

基金资助:
国家自然科学基金(21788102); 广东省自然科学基金(2019B030301003); 以及香港创新科技委员会(ITC-CNERC14SC01)

Recent Advances and Application Prospects in Photothermal Materials^★

He Xu^a^,^b, Pengbo Han^a^,^b, Anjun Qin^a^,^b(), Ben Zhong Tang^b^,^c^,^d

a State Key Laboratory of Luminescent Materials and Devices, Guangdong Provincial Key Laboratory of Luminescence from Molecular Aggregates, South China University of Technology, Guangzhou 510640, China
b Center for Aggregation-Induced Emission, South China University of Technology, Guangzhou 510640, China
c School of Science and Engineering, Shenzhen Institute of Molecular Aggregate Science and Engineering, The Chinese University of Hong Kong, Shenzhen (CUHK-Shenzhen), Guangdong 518172, China
d Hong Kong Branch of Chinese National Engineering Research Centre for Tissue Restoration and Reconstruction, The Hong Kong University of Science & Technology, Clear Water Bay, Kowloon, Hong Kong 999077, China

Received:2023-05-17 Published:2023-07-13
Contact: *E-mail: msqinaj@scut.edu.cn
About author:
^★Dedicated to the 90th anniversary of Acta Chimica Sinica.
Supported by:
National Natural Science Foundation of China(21788102); Natural Science Foundation of Guangdong Province(2019B030301003); Innovation and Technology Commission of Hong Kong(ITC-CNERC14SC01)

Photothermal effect refers to the characteristics of materials that could generate heat under the irradiation of sun or laser light. It can not only maximize the efficiency of solar energy conversion, but also break through the spatiotemporal limitation of laser light transmission, which holds excellent potential and application prospect. Currently, researchers have developed many photothermal materials based on three main photothermal effect mechanisms, plasmonic heating, non-radiative relaxation in semiconductors and thermal vibration in molecules, which include metal nanomaterials, inorganic semiconductor materials, carbon materials, two-dimensional transition metal carbides and nitrides (MXenes), organic small molecules, polymer materials, metal organic framework (MOF), covalent organic framework (COF), organic co-crystals materials, etc. Among them, inorganic materials have the advantages of a wide range of sources, simple structure and excellent thermal stability, while organic materials can be easily designed in structure, and have better biocompatibility. Based on these attractive characteristics, the photothermal effects have been extensively investigated in the area of energy utilization, biomedicine, catalytic conversion, intelligent devices, etc., and realized the applications in photothermal solar evaporation, photothermal therapy, photothermal catalysis, photothermal functional materials. In addition to the rapid development of traditional applications, novel applications have also been explored, such as anti-icing coating, reversible adhesive, agriculture heaters, photothermal energy storage, photothermal induced self-healing materials, photothermal-driven soft robots, etc. However, there are still some challenges in the research of photothermal materials, such as narrow absorption range, low photothermal conversion efficiency, limited application development, and difficulty in use of the elevated temperature induced by photothermal effect. This review briefly summarizes the progresses in the development, utilization of photothermal materials. The challenges and the development direction of photothermal materials are also discussed. It is hope that this review could provide inspiration for the further research in terms of construction of new photothermal materials and innovation of their application.

Key words: photothermal effect, photothermal material, photothermal therapy, photothermal catalysis, photothermal functional device

Cite this article

He Xu, Pengbo Han, Anjun Qin, Ben Zhong Tang. Recent Advances and Application Prospects in Photothermal Materials^★[J]. Acta Chimica Sinica, 2023, 81(10): 1420-1437.

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Fig. & Tab. 14

Figure 1. Mechanism and applications of photothermal effect

Figure 2. Mechanisms of photothermal effect. (a) Plasmonic heating. (b) Non-radiative relaxation in semiconductors. (c) Thermal vibration in molecules

Figure 3. (a) UV-vis absorption spectra of 9, 22, 48, and 99 nm gold nanoparticles in water[15]. Reprinted with permission from Ref. [15], Copyright 1999, American Chemical Society. (b) UV-vis absorption spectra of gold and gold-silver alloy nanoparticles with varying gold mole fractions xAu[21]. (c) Extinction coefficients ε with varying gold mole fractions xAu[21]. Reprinted with permission from Ref. [21], Copyright 1999, American Chemical Society. (d) Absorption of aluminium-based plasmonic absorbers[14]. Reprinted with permission from Ref. [14], Copyright 2016, Springer Nature Limited. (e) Transmittance spectra and (f) photothermal property of TBNWs[22], dispersed in cyclohexane. Reprinted with permission from Ref. [22], Copyright 2018, American Chemical Society

Figure 4. (a) Illustration of the electron-hole generation and relaxation in a normal semiconductor and in narrow-bandgap Ti2O3[23]. Reprinted with permission from Ref. [23], Copyright 2016, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. (b) Scheme of 3D cup structure, which can efficiently recycle the diffuse reflection light and thermal radiation[43]. Reprinted with permission from Ref. [43], Copyright 2018, Elsevier Inc. (c) The corresponding structural models of the hexagonal MoO2 NPs, the sSMO NRs and oxygen-incorporated MoS2 with enlarged interlayer spacing and the photothermal performance of the sSMO NRs-PDMS composite[38]. Reprinted with permission from Ref. [38], Copyright 2017, The Authors, under exclusive license to Springer Nature Ltd. (d) Typical morphologies of the MoO3?x SNW, photothermal performance and shape recovery process of the MoO3?x SNW-PVA film[39]. Reprinted with permission from Ref. [39], Copyright 2021, American Chemical Society

Figure 5. (a) Light absorption spectra of the different wood-based SSGDs[53]. (b) Steam generation digital images of the wood-based SSGDs under light intensities of 5 and 10 suns[53]. Reprinted with permission from Ref. [53], Copyright 2017, Elsevier Inc. (c) Schematic illustration of the photo-electrothermal solar steam generation system with graphene[44]. Reprinted with permission from Ref. [44], Copyright 2018, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. (d) Collecting process of the viscous crude oil by NVGQF (nitrogen-doped vertical graphene which is grown on quartz foam) based on temperature-gradient-driven[54]. Reprinted with permission from Ref. [54], Copyright 2022, American Chemical Society

Figure 7. The illustration of working mechanisms of aggregation-induced emission (AIE) and intramolecular motion-induced photothermy (iMIPT)[73]. Reprinted with permission from Ref. [73], Copyright 2019, The Authors, under exclusive license to Springer Nature Ltd

Figure 8. (a) Schematic illustration of the overall fabrication process toward multilayer PPy nanosheets via sequential polymerization[77]. Reprinted with permission from Ref. [77], Copyright 2019, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. (b) Design of the TCCA-doped PDA NPs. Reprinted with permission from Ref. [78], Copyright 2022, American Chemical Society. (c) Chemical composition and photothermal performance of the LCE material. Reprinted with permission from Ref. [82], Copyright 2017, American Chemical Society. (d) Chemical structure and photothermal performance under 808 nm laser of GS-POP-2[83]. Reprinted with permission from Ref. [83], Copyright 2021, WILEY-VCH GmbH

Figure 9. (a) Representation of the crystalline structure and photothermal performance of the studied MOFs[61]. Reprinted with permission from Ref. [61], Copyright 2018, American Chemical Society. (b) Illustration of the photothermal conversion of Zr-PDI?? and photothermal conversion curves of Zr-PDI?? film[62]. Reprinted with permission from Ref. [62], Copyright 2019, The Authors, under exclusive license to Springer Nature Ltd. (c) Illustration of the sandwich CT complex formation and cocrystallization of TAHC and its solar-thermal conversion[65]. Reprinted with permission from Ref. [65], Copyright 2022, WILEY-VCH GmbH

Figure 10. (a) Synthetic route to TFM and TFM NPs[90]. (b) Illustration of the use of TFM NPs for PAI-guided PTT-PDT cancer theranostics[90]. Reprinted with permission from Ref. [90], Copyright 2019, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. (c) Schematic illustration of state transformation of BTPPA to boost the photothermal conversion efficiency. Reprinted with permission from Ref. [91], Copyright 2021, WILEY-VCH GmbH

Figure 11. (a) Two-step water-based CO2 conversion driven by solar energy[99]. Reprinted with permission from Ref. [99], Copyright 2014, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. (b) Enhancing electrocatalytic water splitting activities via photothermal effect[101]. Reprinted with permission from Ref. [101], Copyright 2019, American Chemical Society. (c) Synthesis NH3 via photothermal catalysis[102]. Reprinted with permission from Ref. [102], Copyright 2019, American Chemical Society. (d) Schematic showing glycolysis of PET in solar thermal catalysis[105]. Reprinted with permission from Ref. [105], Copyright 2022, Elsevier Inc

Figure 12. (a) Solar spectral irradiation across a wavelength range of 300 to 2500 nm[10]. Reprinted with permission from Ref. [10], Copyright 2018, Elsevier Inc. (b) Seawater desalination device based on GS-POP-2-PU and its absorption spectra[83]. Reprinted with permission from Ref. [83], Copyright 2021, WILEY-VCH GmbH. (c) Seawater desalination device based on TPA-TPA-O6 and its water evaporation rate[74]. Reprinted with permission from Ref. [74], Copyright 2022, WILEY-VCH GmbH. (d) Seawater desalination device based on Cu-MOF and its photothermal performance[106]. Reprinted with permission from Ref. [106], Copyright 2021, The Royal Society of Chemistry

Figure 13. The application of photothermal effect under solar. (a) Anti-icing coating[57]. Reprinted with permission from Ref. [57], Copyright 2022, WILEY-VCH GmbH. (b) Energy storage materials[111]. Reprinted with permission from Ref. [111], Copyright 2022, American Chemical Society. (c) Energy conversion[78]. Reprinted with permission from Ref. [78], Copyright 2022, American Chemical Society. (d) Reversible adhesive[109]. Reprinted with permission from Ref. [109], Copyright 2021, WILEY-VCH GmbH

Figure 14. The application of photothermal effect under Laser. (a) Reversible adhesive[110]. Reprinted with permission from Ref. [110], Copyright 2019, American Chemical Society. (b) Photothermal-driven soft robots[114]. Reprinted with permission from Ref. [114], Copyright 2021, WILEY-VCH GmbH. (c) Photothermal induced self-healing materials[112]. Reprinted with permission from Ref. [112], Copyright 2018, The Royal Society of Chemistry

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光热材料的发展现状及应用前景^★

Recent Advances and Application Prospects in Photothermal Materials^★

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光热材料的发展现状及应用前景★

Recent Advances and Application Prospects in Photothermal Materials★

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光热材料的发展现状及应用前景^★

Recent Advances and Application Prospects in Photothermal Materials^★