Review of Theoretical and Applied Research of Graphene in Anti-corrosion Film and Organic Anti-corrosion Coatings

doi:10.6023/A19050174

Acta Chimica Sinica ›› 2019, Vol. 77 ›› Issue (11): 1140-1155.DOI: 10.6023/A19050174 Previous Articles Next Articles

Review

石墨烯在防腐薄膜和有机防腐涂层领域的理论和应用研究综述

丁锐^a^c, 陈思^b, 吕静^a, 桂泰江^d, 王晓^d^e, 赵晓栋^a, 刘杰^a, 李秉钧^a, 宋立英^c^f*(), 李伟华^b^c^f*()

^a 烟台大学海洋学院烟台 264005
^b 中山大学化学工程与技术学院珠海 519082
^c 中国科学院海洋研究所海洋环境腐蚀与生物污损重点实验室青岛 266071
^d 海洋涂料国家重点实验室海洋化工研究院青岛 266071
^e 中国海洋大学青岛 266071
^f 海洋科学与技术国家实验室海洋腐蚀与防护开放工作室青岛 266237

投稿日期:2019-05-13 发布日期:2019-09-24
通讯作者: 宋立英,李伟华 E-mail:songliying@qdio.ac.cn;liweihua@qdio.ac.cn
作者简介:宋立英, 2009年毕业于青岛大学, 获学士学位; 2012年毕业于天津大学, 获硕士学位; 2015年毕业于中国科学院海洋研究所, 获得博士学位; 此后在中国科学院海洋研究所李伟华课题组(2015.08~2017.08)从事博士后研究工作. 2017年9月加入中国科学院海洋研究所海工腐蚀与控制课题组任助理研究员, 主要研究方向为腐蚀产物对金属腐蚀的影响及海洋智能防腐涂层的研究|李伟华, 海洋化学博士, 海洋科学博士后.中山大学化学工程与技术学院院长, 二级教授, 博士生导师.国家杰出青年科学基金获得者, 国家“万人计划”领军人才, 科技部中青年创新领军人才, 中国科学院特聘研究员, 青岛海洋科学与技术试点国家实验室卓越科学家, 德国慕尼黑工业大学高级访问学者, 兼任中国腐蚀与防护学会常务理事, 中国腐蚀与防护学会污损技术专委会副主任, 中国腐蚀与防护学会非金属材料专委会副主任等.主要从事海洋腐蚀与防护方面的研究, 旨在通过不同尺度、多学科交叉的综合手段, 致力于海洋恶劣环境下海工材料腐蚀诱发机理, 功能化防护材料, 以及防御调控新技术的前沿性和创新性研究
基金资助:
国家杰出青年科学基金(51525903);国家自然科学基金面上项目(51179182);中国博士后科学基金面上资助(2018M632726);海洋涂料国家重点实验室开放课题(20190601DR)

Review of Theoretical and Applied Research of Graphene in Anti-corrosion Film and Organic Anti-corrosion Coatings

Ding Rui^a^c, Chen Si^b, Lv Jing^a, Gui Tai-jiang^d, Wang Xiao^d^e, Zhao Xiao-dong^a, Liu Jie^a, Li Bing-jun^a, Song Li-ying^c^f*(), Li Wei-hua^b^c^f*()

^a School of Ocean, Yantai University, Yantai 264005, China
^b College of Chemical Engineering and Technology, Sun Yat-sen University, Zhuhai 519082, China
^c Key Laboratory of Marine Environmental Corrosion and Bio-fouling, Institute of Oceanology, Chinese Academy of Sciences, Qingdao 266071, China
^d Marine Chemical Research Institute, State Key Laboratory of Marine Coatings, Qingdao 266071, China
^e Ocean University of China, Qingdao 266071, China
^f National Laboratory for Marine Science and Technology, Open Studio for Marine Corrosion and Protection, Qingdao 266237, China

Received:2019-05-13 Published:2019-09-24
Contact: Song Li-ying,Li Wei-hua E-mail:songliying@qdio.ac.cn;liweihua@qdio.ac.cn
Supported by:
the National Science Fund for Distinguished Young Scholars(51525903);the National Natural Science Foundation of China(51179182);China Postdoctoral Science Fund(2018M632726);Open Research Fund supported by State Key Laboratory for Marine Coatings(20190601DR)

This paper summarized and collated domestic and foreign literatures on graphene anti-corrosion films and organic anti-corrosion coatings, and formed hierarchical and organized knowledge structures. The preparation, optimization and improvement of graphene anti-corrosion film were reviewed. The corrosion acceleration problems and solutions in the application were discussed. According to the role of graphene in organic anti-corrosion coatings, the improvement of shielding, bonding and self-repairing effect of graphene-based composite materials on organic anti-corrosion coatings are reviewed from the perspective of applied and theoretical research. And the improvement of graphene-based materials on electrochemical protection performance of cathodic-protective organic anti-corrosion coatings are discussed.

Key words: graphene, anti-corrosion, film, coating

Cite this article

Ding Rui, Chen Si, Lv Jing, Gui Tai-jiang, Wang Xiao, Zhao Xiao-dong, Liu Jie, Li Bing-jun, Song Li-ying, Li Wei-hua. Review of Theoretical and Applied Research of Graphene in Anti-corrosion Film and Organic Anti-corrosion Coatings[J]. Acta Chimica Sinica, 2019, 77(11): 1140-1155.

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Fig. & Tab. 12

Figure 1. Graphene film prepared by (a) CVD methods and (b) mechanical transfer methods

Figure 2. Relationship between the layers number of graphene film and the corrosion inhibition effect

Figure 3. Corrosion protection mechanism of graphene film and the corrosion promotion mechanism in defect area

Figure 4. Improved method of graphene film. (a) Multilayer stacking and (b) atomic layer deposition

Figure 5. Inductive research content of graphene organic anti-corrosion coatings

Figure 6. Graphene dispersion methods

Figure 7. Summary of graphene dispersion methods. (a, b) Unmodified dispersion, (c~e) chemical modification dispersion and (f~h) physical adsorption dispersion

Figure 8. Covalent bonding of p-phenylenediamine/4-vinylbenzoic acid modified graphene to polystyrene

Figure 9. In situ polymerization preparation technology of graphene/polyaniline composite

Figure 10. Orientation methods of graphene. (a) Magnetic field induction, (b) electric field induction and (c) layer-by-layer self-assembly

Figure 11. Functionalization of graphene. (a) Enhanced coating adhesion, (b) self-healing based on catalytic passivation, and (c) self-healing based on corrosion inhibitor

Figure 12. Mechanism of graphene modified zinc-rich coatings. (a) Macroscopic barrier kinetics, (b) mesoscopic electrochemical structure and transmission line model and (c) microscopic quantum mechanical mechanism of electronic transmission

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石墨烯在防腐薄膜和有机防腐涂层领域的理论和应用研究综述

Review of Theoretical and Applied Research of Graphene in Anti-corrosion Film and Organic Anti-corrosion Coatings

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