Research Progress in the Synthesis and Properties of Chiral Metal-Organic Frameworks★

doi:10.6023/A26020039

Acta Chimica Sinica ›› 2026, Vol. 84 ›› Issue (5): 723-735.DOI: 10.6023/A26020039 Previous Articles Next Articles

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手性金属-有机框架的合成与性质研究进展^★

孙天凯, 韩宗甦, 程鹏, 师唯^*()

南开大学化学学院天津 300071

投稿日期:2026-02-01 发布日期:2026-04-14
通讯作者: 师唯

作者简介:

孙天凯, 博士研究生. 2019年毕业于南开大学(分子科学与工程专业), 获理学学士和工学学士学位. 2019年起在南开大学化学学院攻读博士学位. 主要研究方向为手性金属-有机框架的设计及其在对映异构体识别中的应用.

韩宗甦, 2016年在南开大学化学学院获理学学士学位, 2022年在南开大学化学学院获理学博士学位. 主要研究方向为金属-有机框架的孔道编辑工程及其在荧光识别中的应用.

程鹏, 南开大学化学学院教授, 博士生导师, 教育部“长江学者”计划特聘教授, 国家自然科学基金杰出青年科学基金获得者. 主要从事配位化学相关的研究工作.

师唯, 南开大学化学学院教授, 博士生导师, 入选教育部新世纪优秀人才支持计划, 国家自然科学基金优秀青年科学基金获得者. 主要从事功能配合物化学相关的研究工作.

★ “框架材料化学”专辑.

基金资助:
国家自然科学基金(22471130)

Research Progress in the Synthesis and Properties of Chiral Metal-Organic Frameworks^★

Tiankai Sun, Zongsu Han, Peng Cheng, Wei Shi^*()

College of Chemistry, Nankai University, Tianjin 300071, China

Received:2026-02-01 Published:2026-04-14
Contact: Wei Shi
About author:
★ For the VSI “Chemistry of Framework Materials”.
Supported by:
National Natural Science Foundation of China(22471130)

Chiral metal-organic frameworks, as a class of advanced chiral materials with highly tunable structures, exhibit promising applications in the fields of medicine, biology, optics and so on. Recently, significant progresses of chiral metal- organic frameworks have been achieved. However, with the interdisciplinary intersection and integration of relevant research and various fields, new challenges have emerged, such as the efficient synthesis of chiral ligands and chiral metal-organic frameworks, their stability in potential application scenarios, and the molecular-level mechanisms underlying their enantioselective applications. This review discusses the direct synthetic strategies of chiral metal-organic frameworks (direct synthesis based on chiral ligands, spontaneous resolution from achiral ligands, chiral template induction, and chiral defect engineering) as well as post-synthetic modification strategies (post-modification of metal ion nodes/organic ligands and post-modification of functional guests). Furthermore, this review summarizes the research advances of chiral metal-organic frameworks in enantioselective sensing, enantiomers separation, asymmetric catalysis, and chiral optics in recent five years, and provides an outlook in the future development of this field.

Key words: metal-organic framework, chirality, synthetic strategy, enantioselective application

Cite this article

Tiankai Sun, Zongsu Han, Peng Cheng, Wei Shi. Research Progress in the Synthesis and Properties of Chiral Metal-Organic Frameworks^★[J]. Acta Chimica Sinica, 2026, 84(5): 723-735.

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Fig. & Tab. 9

Figure 1. The search results for “chiral metal-organic frameworks” in Web of Science

Figure 2. The synthetic strategies for chiral metal-organic frameworks

Figure 3. (A) Arrangements of organic ligands around the Ni(II) centers in chiral 2D MOF, 1P and 1M. (B) The helical structure of 1M and 1P. (C) Absolute configurations around Ni(II) centers in the 1M and 1P. (D) Structures of 2D→3D parallel interpenetration. Reprinted with permission from ref. [38], Copyright 2025 Wiley-VCH

Figure 4. (A) Synthetic route for chiral defective metal-organic frameworks. (B) Pore size distribution and acid-base stability and (C) structures of four schematic diagrams of defective metal-organic frameworks. Reprinted with permission from ref. [41], Copyright 2023 Elsevier Publishing Group

Figure 6. Ion exchange of Zn-MOF. First step: the replacement of (CH3)2NH2＋ with N-benzylquininium cations. Second step: the lead-in of Tb3＋. Reprinted with permission from ref. [48], Copyright 2019 The Authors

Figure 7. (A) Sensing of ee values of I/II-C-Tb towards enantiomeric mixtures. (B) Enantioselective sensing mechanism of I/II-C-Tb. Reprinted with permission from ref. [52], Copyright 2022 Wiley-VCH

Figure 8. (A) Molecular structures of H4L1 and H4L2. (B) 8- and 12-connected Zr6 clusters in CMOF-1 and CMOF-2. (C) 3D structures of CMOF-1 and CMOF-2; (D) Dumbbell-like cavities in CMOF-1 and CMOF-2. Reprinted with permission from ref. [12], Copyright 2022 American Chemical Society

Figure 9. The design and construction of the solution-processable MOF system featuring highly dynamic aggregation states by utilizing the highly reversible and dynamic features of coordination bonding, and the features of stimuli-responsive luminophore originated from dynamic aggregation tuning. Reprinted with permission from ref. [64], Copyright Copyright 2025 Wiley-VCH

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手性金属-有机框架的合成与性质研究进展^★

Research Progress in the Synthesis and Properties of Chiral Metal-Organic Frameworks^★

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手性金属-有机框架的合成与性质研究进展★

Research Progress in the Synthesis and Properties of Chiral Metal-Organic Frameworks★

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手性金属-有机框架的合成与性质研究进展^★

Research Progress in the Synthesis and Properties of Chiral Metal-Organic Frameworks^★