有机化学 ›› 2018, Vol. 38 ›› Issue (8): 1917-1929.DOI: 10.6023/cjoc201803021 上一篇    下一篇

综述与进展

氮掺杂碳材料负载Pd纳米催化剂在有机反应中的最新研究进展

李晓微a,b, 许海芬a, 周晋a, 闫格a, 张雷b,c, 禚淑萍a   

  1. a 山东理工大学化学化工学院 淄博 255000;
    b 南京大学配位化学国家重点实验室 南京 210023;
    c 安徽理工大学材料科学与工程学院 淮南 232001
  • 收稿日期:2018-03-15 修回日期:2018-04-23 发布日期:2018-05-03
  • 通讯作者: 张雷, 禚淑萍 E-mail:yutian1224@126.com;zhuosp_academic@yahoo.com
  • 基金资助:

    国家自然科学基金(Nos.51502162,21501002,21576159)、南京大学配位化学国家重点实验室开放课题(Nos.SKLCC1613,SKLCC1604)、中国科学院光化学转化与功能材料重点实验室(理化技术研究所)开放课题(No.PCOM201704)、国家级大学生创新训练计划(No.201710433179)和山东理工大学青年教师发展支持计划资助项目.

Recent Progress of N-Doped Carbon Materials Supported Pd Nanocatalysts in Organic Reactions

Li Xiaoweia,b, Xu Haifena, Zhou Jina, Yan Gea, Zhang Leib,c, Zhuo Shupinga   

  1. a School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo 255000;
    b State Key Laboratory of Coordination Chemistry, Nanjing University, Nanjing 210023;
    c School of Materials Science and Engineering, Anhui University of Science and Technology, Huainan 232001
  • Received:2018-03-15 Revised:2018-04-23 Published:2018-05-03
  • Contact: 10.6023/cjoc201803021 E-mail:yutian1224@126.com;zhuosp_academic@yahoo.com
  • Supported by:

    Project supported by the National Natural Science Foundation of China (Nos. 51502162, 21501002, 21576159), the Open Foundation of State Key Laboratory of Coordination Chemistry of Nanjing University (Nos. SKLCC1613, SKLCC1604), the Open Fund of Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, the Chinese Academy of Sciences (No. PCOM201704), the National Students' Innovation Training Program (No. 201710433179) and the Young Teacher Supporting Fund of Shandong University of Technology.

氮掺杂碳材料负载Pd纳米催化剂因其具有反应活性高、反应完成后便于分离和重复使用等优点,在催化领域引起了极为广泛的关注.简要综述了基于氮掺杂多孔/介孔碳NC、氮掺杂石墨烯NG、氮掺杂碳纳米管NCNT和氮掺杂碳纳米片NCNS等不同类型碳材料载体制备的负载型Pd纳米催化剂的合成与应用的最新研究进展,同时对氮掺杂碳材料负载Pd纳米催化剂的发展方向进行了展望.

关键词: 氮掺杂碳材料, 负载, Pd纳米催化剂, 有机反应

The N-doped carbon materials supported Pd nanocatalysts have attracted extensive attention in the catalysis field due to its unique advantages such as high efficiency, easy separation, purification and recyclability. The recent progress in the synthesis and application of supported Pd nanocatalysts based on different types of carbon materials supports including N-doped porous/mesoporous carbon, N-doped graphene, N-doped carbon nanotube and N-doped carbon nanosheet is reviewed. And the research trends of N-doped carbon materials supported Pd nanocatalysts are also prospected.

Key words: N-doped carbon material, support, Pd nanocatalyst, organic reaction