光热材料在海水淡化领域的近期研究进展与展望★

doi:10.6023/A23040148

化学学报 ›› 2023, Vol. 81 ›› Issue (8): 1052-1063.DOI: 10.6023/A23040148 上一篇下一篇

所属专题：庆祝《化学学报》创刊90周年合辑

综述

光热材料在海水淡化领域的近期研究进展与展望^★

杨地^a, 史潇凡^b, 张冀杰^a^,^*(), 卜显和^a^,^c

a 南开大学材料科学与工程学院金属与分子基材料化学天津市重点实验室天津 300350
b 武汉大学化学与分子科学学院生物医学高分子材料教育部重点实验室武汉 430072
c 南开大学化学学院元素有机化学国家重点实验室天津 300071

投稿日期:2023-04-20 发布日期:2023-09-14

作者简介:

杨地, 1998年出生于河南镇平, 2017年毕业于桂林理工大学, 获学士学位. 目前在卜显和教授指导下攻读硕士学位. 研究兴趣为光催化水分解产氢.

史潇凡, 1997年出生于安徽合肥, 2019年毕业于南京航空航天大学, 获学士学位. 2022年毕业于南开大学, 获材料工程硕士学位, 导师为卜显和教授. 现于武汉大学攻读无机化学博士学位, 导师为邓鹤翔教授. 研究方向为MOF基光催化剂的合成与性能研究.

张冀杰, 2012年和2018年在天津大学获得学士和博士学位. 2018年至今在南开大学材料科学与工程学院卜显和院士课题组从事博士后研究. 主要研究领域涉及功能金属有机框架材料的设计构筑和太阳能催化转化反应过程中的机理研究.

卜显和, 教授、博导、国家杰青、长江学者、天津市首批杰出人才、全国政协委员、英国皇家化学会会士、南开大学材料科学与工程学院院长、中国科学院院士. 在配位聚合物的功能导向构筑、结构调控及性能研究等方面取得了系统成果.

^★庆祝《化学学报》创刊90周年.

基金资助:
项目受国家自然科学基金(21908113); 天津市应用基础研究项目(21JCYBJC00140)

Recent Research Progress and Prospect of Photothermal Materials in Seawater Desalination^★

Di Yang^a, Xiaofan Shi^b, Jijie Zhang^a(), Xian-He Bu^a^,^c

a Tianjin Key Laboratory of Metal and Molecule-Based Material Chemistry, School of Materials Science and Engineering, Nankai University, Tianjin 300350
b Key Laboratory of Biomedical Polymers of Ministry of Education, College of Chemistry and Molecular Science, Wuhan University, Wuhan 430072
c State Key Laboratory of Elemento-Organic Chemistry, College of Chemistry, Nankai University, Tianjin 300071

Received:2023-04-20 Published:2023-09-14
Contact: *E-mail: zhangjijie@nankai.edu.cn
About author:
^★Dedicated to the 90th anniversary of Acta Chimica Sinica.
Supported by:
National Natural Science Foundation of China(21908113); Tianjin Applied Basic Research Project(21JCYBJC00140)

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摘要/Abstract

太阳能水蒸发系统成本低、能效高, 对缓解能源危机、减少水污染、促进海水淡化具有重要意义. 然而, 太阳能驱动水蒸发的自然机制往往受到低蒸发率和吸收光谱范围小的影响. 其中, 局部加热并限制热损失的界面水蒸发策略被广泛认可并作为高性能、可持续的太阳能蒸汽产生的有效途径. 随着太阳能水蒸发技术的不断发展, 制备绿色、高效的光热材料已成为研究热点. 根据光热材料的种类将其划分为: 金属材料、半导体材料、碳基材料以及聚合物材料, 详细阐述了不同材料的光热转换机制并总结近年来光热材料在海水淡化领域的研究现状及进展; 讨论了潜在的光热候选材料, 对其未来发展做出了展望. 旨在为海水淡化领域中高效光热材料的合理设计和开发提供可行方案, 对今后光热材料的发展具有总结和指导意义.

关键词: 海水淡化, 光热材料, 界面蒸发

Solar water evaporation system has appealing advantages of low cost and high energy efficiency, which is of great significance to alleviate energy crisis, reduce water pollution and promote seawater desalination. However, the natural mechanism of solar-driven water evaporation system is often affected via low evaporation rate and small absorption spectrum range. The interface evaporation strategy that locally heats and limits heat loss is widely recognized as a high-performance and sustainable approach for efficient solar steam generation. With the continuous development of solar evaporation technology, the preparation of green and efficient photothermal materials has become a research hotspot. In this review, the photothermal materials were classified into metal materials, semiconductor materials, carbon-based materials and polymer materials according to their types. It elaborated on the photothermal conversion mechanisms of different materials and summarized the research status and progress of photothermal materials in the field of seawater desalination in recent years. The potential candidate photothermal materials were discussed and their future development was forecasted. This review aims to propose practical strategies for the rational design and development of efficient photothermal materials in the field of seawater desalination. The findings summarized in this review are of great significance for the future development of photothermal materials and provide valuable guidance for future research in this area.

Key words: seawater desalination, photothermal material, interfacial evaporation

引用此文

杨地, 史潇凡, 张冀杰, 卜显和. 光热材料在海水淡化领域的近期研究进展与展望^★[J]. 化学学报, 2023, 81(8): 1052-1063.

Di Yang, Xiaofan Shi, Jijie Zhang, Xian-He Bu. Recent Research Progress and Prospect of Photothermal Materials in Seawater Desalination^★[J]. Acta Chimica Sinica, 2023, 81(8): 1052-1063.

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图/表 10

图1. 界面太阳能蒸发器示意图

Figure 1. Figure caption schematics of solar interfacial evaporators Repriented (Adapted or Reprinted in part) with permission from {ACS Energy. Lett. 2023, 8, 1680.}. ? {2023} American Chemical Society.

图2. 实际阳光照射下太阳能驱动海水淡化试验的光学照片

Figure 2. The optical photographs of the solar-driven desalination test under the actual sunlight irradiation Reprinted (Adapted or Reprinted in part) with permission from {ACS Nano 2022, 16, 2511.}. ? {2022} American Chemical Society

图3. 光热效应原理示意图

Figure 3. Schematic diagram of the photothermal effect principle Reprinted (Adapted or Reprinted in part) with permission from {ACS Appl. Polym. Mater. 2020, 2, 4273.}. ? {2020} American Chemical Society.

图4. 各类光热材料的光热机制

Figure 4. The photothermal mechanisms of various types of photothermal materials

图5. 近年间具有代表性的光热材料研究工作水蒸发速率及光热转换效率图

Figure 5. Water evaporation rate and photothermal conversion efficiency diagram of representative photothermal materials research work in recent years

样品	光强/(kW•m^－2)	水蒸发速率/(kg•m^－2•h^－1)	光热转换效率/%	参考文献
Au纳米颗粒(3.4 nm)	1	—	11	[48]
Au纳米颗粒(37.7 nm)	1	—	30	[48]
Au/MCE	10	—	85	[49]
Ag纳米颗粒薄膜	1	1.37	89.3	[51]
AuF	1	—	85	[52]
Ti₂O₃	1	1.32	—	[28]
Li₂TiO₃	2	0.87	—	[56]
MoN/Mo₂N	1	1.7	98	[58]
V/MoO₃	1	2.0	93.44	[59]
Ni₃S₂/NF	1	1.29	87.2	[60]
Co₃O₄/Ni	1	1.226	80	[61]
C, N-TiO₂纳米片@Ti板	1	1.57	—	[62]
CNPs/PDMS/PVA	0.85	1.26	80	[64]
F-Wood	1	—	72	[68]
2D C/Cu	1	—	65	[75]
N/3D rGO	1	—	80	[77]
3DGN/Wood	1	—	91.8	[78]
SPPU@NCS	1	2.18	—	[79]
HPCNFs	1	1.78	96.13	[80]
PPy-Wood	1	1.014	72.5	[84]
聚吡咯-木棉纤维气凝胶	1	—	82.4	[85]
聚乙烯醇/聚吡咯/壳聚糖	1	3.6	—	[86]
BPF	5	0.57	48.3	[87]
聚酰亚胺/MXene	5	—	50.6	[88]
PFF	1	1.48	87.4	[90]
PPY/BTA	1	1.90	89	[91]

表1. 光热材料的性能参数

Table 1. Performance parameters of photothermal materials

图6. 在空气-水界面自组装的金纳米颗粒的浮动等离子体膜辅助下液体的有效蒸发示意图

Figure 6. Schematic illustration of efficient evaporation of liquid assisted by a floating plasmonic film of gold nanoparticles self-assembled at the air-water interface Reprinted (Adapted or Reprinted in part) with permission from {Small 2014, 10, 3234.}. ? {2014} John Wiley and Sons.

图7. 太阳能蒸发示意图

Figure 7. Solar evaporation diagram Reprinted (Adapted or Reprinted in part) with permission from {ACS Mater. Lett. 2022, 4, 1584.}. ? {2022} American Chemical Society.

图8. 基于3DGN的太阳能海水淡化装置的(a)3DGN制造过程和(b)工作过程示意图; 插图显示了3DGN介孔结构中光的多次散射和气泡的形成

Figure 8. Schematic of (a) 3DGN fabrication procedure and (b) working process of the 3DGN-based solar desalination device; the right inset shows multiple scattering of light and the formation of water bubbles in the mesoporous structure of 3DGN Reprinted (Adapted or Reprinted in part) with permission from {ACS Appl. Mater. Inter. 2018, 10, 15602.}. ? {2018} American Chemical Society.

图9. Cu-CAT-1 MOF光催化剂的制备示意图

Figure 9. Schematic illustration of the construction of Cu-CAT-1 MOF photocatalysts Reprinted (Adapted or Reprinted in part) with permission from {Adv. Mater. 2019, 31, 1808249.}. ? {2019} John Wiley and Sons.

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光热材料在海水淡化领域的近期研究进展与展望^★

Recent Research Progress and Prospect of Photothermal Materials in Seawater Desalination^★

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光热材料在海水淡化领域的近期研究进展与展望★

Recent Research Progress and Prospect of Photothermal Materials in Seawater Desalination★

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光热材料在海水淡化领域的近期研究进展与展望^★

Recent Research Progress and Prospect of Photothermal Materials in Seawater Desalination^★