Functionalized Carbon-Based Composite Materials for Cathode Application of Lithium-Sulfur Batteries

doi:10.6023/A21080381

Acta Chimica Sinica ›› 2022, Vol. 80 ›› Issue (1): 89-97.DOI: 10.6023/A21080381 Previous Articles Next Articles

Review

功能碳基复合材料在锂硫电池正极中的应用

刘汉鼎^a^,^b, 贾国栋^b, 朱胜^b, 盛建^b, 张则尧^a^,^b, 李彦^a^,^b^,^*()

^a北京大学深圳研究院深圳 518057
^b北京分子科学国家研究中心纳米器件物理与化学教育部重点实验室稀土材料及应用国家重点实验室北京大学化学与分子工程学院北京 100871

投稿日期:2021-08-14 发布日期:2021-11-12
通讯作者: 李彦

作者简介:

刘汉鼎, 目前在北京大学化学与分子工程学院李彦教授课题组开展研究工作, 研究方向是碳纳米管及其衍生物的可控制备及在储能领域的应用研究.

李彦, 北京大学化学与分子工程学院教授, 主要从事碳纳米材料的研究, 在碳纳米管的可控生长、分离、表征和应用等方面取得了一系列重要研究成果. 2011年获得国家杰出青年基金资助, 2013年获聘教育部长江学者特聘教授, 以第一完成人获2017年度教育部自然科学一等奖.

基金资助:
深圳市科技计划项目(JCYJ20170817113121505); 深圳市海外高层次人才创新创业专项资金(KQTD20180411143400981); 科技部国家科技重大专项(2016YFA0201904); 国家自然科学基金(21631002); 国家自然科学基金(52101209); 北京分子科学国家研究中心(BNLMS-CXTD-202001); 中国博士后面上基金项目(2020M682606)

Functionalized Carbon-Based Composite Materials for Cathode Application of Lithium-Sulfur Batteries

Handing Liu^a^,^b, Guodong Jia^b, Sheng Zhu^b, Jian Sheng^b, Zeyao Zhang^a^,^b, Yan Li^a^,^b()

^aPeking University Shenzhen Institute, Shenzhen 518057, China
^bBeijing National Laboratory for Molecular Science, Key Laboratory for the Physics and Chemistry of Nanodevices, State Key Laboratory of Rare Earth Materials Chemistry and Applications, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China

Received:2021-08-14 Published:2021-11-12
Contact: Yan Li
Supported by:
Shenzhen Basic Research Project(JCYJ20170817113121505); Shenzhen KQTD Project(KQTD20180411143400981); National Science and Technology Major Project of the Ministry of Science and Technology of China(2016YFA0201904); National Natural Science Foundation of China(21631002); National Natural Science Foundation of China(52101209); Beijing National Laboratory for Molecular Sciences(BNLMS-CXTD-202001); China Postdoctoral Science Foundation(2020M682606)

Carbon-based materials exhibit excellent physical and chemical properties due to their diverse structure, adjustable morphology and controllable composition. They have great application potentials in the field of new energy storage and conversion. Lithium-sulfur batteries as a kind of important new energy storage devices are trapped by the sulfur and lithium sulfide bottleneck of electronic insulation, which leads to irreversible charging and discharging processes. Fortunately, carbon-based composite materials have strong electrical conductivity. The coupling of multi-functions of the composite materials can improve the long-term utilization of sulfur and alleviate the attenuation of cycle and rate capacity. Functionalized carbon-based composite materials can be prepared through surface/interface and defect engineering techniques, which have attracted the attention and favor of scientific researchers. We review the preparation methods of functionalized carbon-based host materials and analyze the structure-function relationship of carbon-based composite materials and sulfur cathodes. We discuss the influence of the change of morphology, structure, and composition on the electrochemical performance of sulfur cathode. Finally, the feasibility of the functionalized carbon-based composite materials are prospected in the practical application of the lithium-sulfur battery.

Key words: carbon-based composite material, lithium-sulfur battery, functional, cathode

Cite this article

Handing Liu, Guodong Jia, Sheng Zhu, Jian Sheng, Zeyao Zhang, Yan Li. Functionalized Carbon-Based Composite Materials for Cathode Application of Lithium-Sulfur Batteries[J]. Acta Chimica Sinica, 2022, 80(1): 89-97.

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Fig. & Tab. 8

Figure 1. Tri-functional design and application of an advanced carbon- based composite sulfur storage host

Figure 2. Schematic illustration of the S/FLHPC composite preparation[47]

Figure 3. Constraint schematic diagram of two-dimensional carbon-based composite host on the functionalization for sulfur cathode[54]

Figure 4. Schematic illustration of the reverse microemulsion method: (a) preparing microemulsion-1, (b) preparing microemulsion-2, and (c) synthesis of sulfur/graphene composite[55]

Figure 5. (a) Synthesis of the MnO2@HCF/S composite, (b) advantages of the MnO2@HCF/S composite over HCF/S[58]

Figure 6. (a) Schematic of the synthetic procedure of the S/YSC@Fe3O4 composite, (b) SEM images of YSC@Fe3O4, (c, d) cyclic performance of S/YSC@Fe3O4 composite cathode with different sulfur load[61]

Figure 7. (a) Energy profiles for the reduction of LiPS on N/G and Co-N/G substrates, (b, c) energy profiles of the decomposition of Li2S cluster on N/G and Co-N/G, electrochemical performance of S@Co-N/G cathode: (d) discharge-charge profiles, (e) rate capabilities[80]

Figure 8. The catalytic mechanism of the LiPS on the surface of Ni@NG in electrochemical process[82]

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功能碳基复合材料在锂硫电池正极中的应用

Functionalized Carbon-Based Composite Materials for Cathode Application of Lithium-Sulfur Batteries

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