共价有机框架的设计及其在催化C—H活化领域的应用进展
收稿日期: 2024-12-06
修回日期: 2024-12-25
网络出版日期: 2025-01-24
基金资助
国家自然科学基金(52270039); 国家自然科学基金(22408149); 江西省研究生创新专项基金(YC2023-006)
Advances in Design of Covalent Organic Frameworks and Their Application in Catalytic C—H Activation
Received date: 2024-12-06
Revised date: 2024-12-25
Online published: 2025-01-24
Supported by
National Natural Science Foundation of China(52270039); National Natural Science Foundation of China(22408149); Jiangxi Provincial Graduate Innovation Special Fund(YC2023-006)
共价有机框架(COFs)作为新兴多孔材料, 因其独特的可设计性、较高的孔隙度和结晶度以及可修饰的孔道环境, 有望成为催化领域中一种重要的催化剂. 近年来, 随着对COFs材料研究的逐渐深入, 人们对其结构设计更为多样化, 逐渐探索出多种有关COFs材料的构建策略, 使其在催化领域中展现出非凡的应用前景. 因此, 从COFs材料的基本结构出发, 全面地讨论了常见的构建策略, 并列举部分COFs材料在C—H活化领域的实际应用, 详细介绍其在这些反应中的催化机理. 最后, 讨论了COFs材料当前在催化领域面临的问题与困境, 期望为COFs材料在催化C—H活化领域未来的发展提供有益指导.
王轩 , 柳茂陈 , 钟瑶 , 宋仁杰 . 共价有机框架的设计及其在催化C—H活化领域的应用进展[J]. 有机化学, 2025 , 45(2) : 448 -465 . DOI: 10.6023/cjoc202410015
Covalent organic frameworks (COFs) are emerging as significant porous materials in the field of catalysis, owing to their unique designability, high porosity, favorable crystallinity, and customizable pore environments. Recent advancements in COFs research have led to increased structural diversity and the exploration of various construction strategies, showcasing their remarkable application prospects in catalysis. This paper offers a comprehensive overview of common strategies employed in constructing COFs based on their fundamental structures. Additionally, several practical applications of COFs in C—H activation are highlighted, elucidating the catalytic mechanisms involved in these reactions. Finally, the current challenges and issues confronting COFs in the realm of catalysis are explored, intending to provide valuable guidance for their future development in C—H activation.
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