Rational Design and Applications of Porous Aromatic Frameworks Photocatalytic Materials

doi:10.6023/A26040102

Acta Chimica Sinica ›› 2026, Vol. 84 ›› Issue (9): 1534-1546.DOI: 10.6023/A26040102 Previous Articles

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多孔芳香骨架光催化材料的合理设计与应用

辛翠^a, 邵京京^b, 何禹萱^b, 陶鑫^b^,^*()

^a 湖南警察学院食药环及毒品检验技术湖南省普通高等学校重点实验室食药环及毒品检验技术湖南省普通高等学校重点实验室长沙 410138
^b 东北师范大学化学学院多酸与网格材料化学教育部重点实验室多酸与网格材料化学教育部重点实验室长春 130024

投稿日期:2026-04-03 发布日期:2026-06-02
通讯作者: 陶鑫

作者简介:

辛翠, 湖南警察学院刑事科学技术系讲师, 主要研究方向为功能材料的合成及在法庭科学领域的应用.

邵京京, 就读于东北师范大学化学学院, 2023级无机化学硕士研究生, 主要研究方向为面向光催化应用的多孔芳香骨架材料的设计与合成.

何禹萱, 就读于东北师范大学化学学院, 2023级无机化学硕士研究生, 主要研究方向为面向光催化应用的多孔芳香骨架材料的设计与合成.

陶鑫, 东北师范大学化学学院教授. 2014年于吉林大学获理学博士学位. 2014~2019年期间, 先后在中国科学院长春应用化学研究所及德国明斯特大学从事博士后研究. 目前主要研究方向为面向能源与环境催化的新型多孔有机材料合成.

基金资助:
国家自然科学基金(52173195); 吉林省科学技术厅(20260102135JC)

Rational Design and Applications of Porous Aromatic Frameworks Photocatalytic Materials

Cui Xin^a, Jingjing Shao^b, Yuxuan He^b, Xin Tao^b^,^*()

^a Key Laboratory of Food & Environment & Drug Monitoring and Testing of Universities in Hunan Province, Hunan Police Academy, Changsha 410138, China
^b Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education, Faculty of Chemistry, Northeast Normal University, Changchun 130024, China

Received:2026-04-03 Published:2026-06-02
Contact: Xin Tao
Supported by:
The National Natural Science Foundation of China(52173195); The Jilin Provincial Department of Science and Technology(20260102135JC)

Photocatalytic technology, renowned for its environmental friendliness, mild reaction conditions, low operational cost, and facile synthetic accessibility, has emerged as one of the most compelling green technologies in modern society. It exhibits promising prospects for practical applications across a broad spectrum of application fields, including atmospheric pollutant abatement, wastewater treatment, aquatic environmental remediation, clean hydrogen evolution, renewable energy conversion, organic synthesis, and green chemical transformation. By harnessing solar energy as the primary driving force, photocatalysis enables the efficient catalytic transformations, successfully achieving storage and conversion of solar energy into chemicals. This strategy is well aligned with the goals of carbon neutrality and sustainable social development. Porous aromatic frameworks (PAFs) represent an innovative category of organic porous materials with broad application prospects. They possess distinctive advantages including precisely tunable topological structures at the molecular level, robust stable covalent linkages, ultra-high specific surface area and favorable porosity, as well as excellent chemical and thermal stability under harsh environments. Meanwhile, PAFs incorporated with diverse photoactive units also exhibit superior light-harvesting capacity across a broad light spectrum, abundant exposed active sites and extended conjugated skeleton structures, thus serving as a promising platform for fabricating high-performance and long-term high-stability photocatalysts. Thus, rationally designing and constructing functional PAFs with adjustable bandgaps, regulated energy levels and efficient photogenerated charge carrier separation and migration, as well as extensively exploring their diverse photocatalytic applications, are of great theoretical and practical significance for linking the internal structure and photocatalytic performance of advanced porous organic semiconductor photocatalysts. The latest research progress and representative achievements of PAFs in the field of photocatalysis are systematically summarized, focusing on their molecular and structural design strategies, photocatalytic reaction mechanisms, diverse application scenarios, as well as existing challenges and future development directions. It aims to provide solid theoretical guidance and valuable practical references for the subsequent development and fabrication of high-performance PAF-based semiconductor photocatalysts.

Key words: photocatalysis, porous aromatic framework, application progress

Cite this article

Cui Xin, Jingjing Shao, Yuxuan He, Xin Tao. Rational Design and Applications of Porous Aromatic Frameworks Photocatalytic Materials[J]. Acta Chimica Sinica, 2026, 84(9): 1534-1546.

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Fig. & Tab. 14

Figure 1. General mechanism of photocatalysis

Figure 2. Applications of photocatalysis

Figure 3. (A) Common coupling reactions in the synthesis of PAFs and (B) PAFs materials used in photocatalytic reactions

Figure 4. Mechanism of photocatalytic H2O2 production

Figure 5. (A) Synthetic routes, (B) HOMO and LUMO, (C) HOMO and LUMO with optimal O2 adsorption in the presence of an electron of COTh-PAFs, and (D) Gibbs free energy diagram for the reduction of O2 to H2O2 on the PAF-363

Figure 6. Schematic diagram of the mechanism by which PAF-370 produces H2O2 via photocatalysis

Figure 7. (A) Synthetic routes of AQ-PAFs, (B) optimal adsorption sites and configurations of O2 on AQ-PAFs, (C) water contact angles of AQ-PAFs, (D) interaction energies of hydrogen bonding between H2O and AQ fragments on the surface of AQ-PAFs, (E) Mulliken atomic charges and the corresponding dipole moments of AQ‑PAFs, (F) dispersion photos of PAF-379 particles in water in various concentrations, and (G) particle size distributions of water suspension of PAF-379 particles in various concentrations

Figure 8. Application of PAFs as catalysts in photocatalytic organic transformations

Figure 9. (A) High-efficiency photosynthesis of 1O2 along the energy transfer pathway via COTh-PAFs photocatalysis, (B) mechanisms of photoinduced charge transfer and energy transfer, (C) MPP and SDP (the blue (red) color intensity corresponds to the displacement below (above) the fitting plane of atom), (D) π-electron localization map, (E) total-SOC of COTh-PAFs, (F) radar plot and (G) adsorption energy of COTh-PAFs

Figure 10. (A) Preparation of Au single-atom catalysts supported on PAF-164 using pre-metallized building blocks, (B) comparative Gibbs free energy profiles for photocatalytic hydrogen evolution over Au5%-SAs-PAF-164 and Au100%-SAs-PAF-164, the geometric structure of (C) pristine Au5%-SAs-PAF-164, (D) Au5%-SAs-PAF-164 after H adsorption, (E) pristine Au100%-SAs-PAF-164 and (F) Au100%-SAs-PAF-164 following H atom adsorption

Figure 11. PAF-332-DCM for near-infrared photocatalytic CO2 reduction

Figure 12. TEPE-TB-PAF for efficient photocatalytic CO₂ reduction

Figure 13. Schematic diagram of photocatalytic degradation of rhodamine B by CQDs/PAF-45

Figure 14. PAF-TPE for efficient degradation of organic pollutants

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多孔芳香骨架光催化材料的合理设计与应用

Rational Design and Applications of Porous Aromatic Frameworks Photocatalytic Materials

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