NMR Studies on Interactions between Oxalate-oxodiperoxovanadate and Arginine

Acta Chimica Sinica ›› 2004, Vol. 62 ›› Issue (3): 230-235. Previous Articles Next Articles

NMR研究草酸双过氧钒配合物与精氨酸的相互作用

曾碧榕¹, 于贤勇¹, 蔡淑惠², 陈忠^1,2, 万惠霖¹

1. 厦门大学化学系固体表面物理化学国家重点实验室, 厦门, 361005;
2. 厦门大学物理系, 厦门, 361005

投稿日期:2003-11-24 修回日期:2003-12-30 发布日期:2014-01-26
通讯作者: 陈忠,E-mail:chenz@jingxian.xmu.edu.cn E-mail:chenz@jingxian.xmu.edu.cn
基金资助:
国家自然科学基金(Nos.10234070,10005006,10104011)和固体表面物理化学国家重点实验室资助项目.

NMR Studies on Interactions between Oxalate-oxodiperoxovanadate and Arginine

ZENG Bi-Rong¹, YU Xian-Yong¹, CAI Shu-Hui², CHEN Zhong^1,2, WAN Hui-Lin¹

1. Department of Chemistry, State Key Laboratory for Physical Chemistry of Solid Surface;
2. Department of Physics, Xiamen University, Xiamen 361005

Received:2003-11-24 Revised:2003-12-30 Published:2014-01-26

Abstract

Coordination interactions between oxalate-oxodiperoxovanadate {K₃[VO(O₂)₂(C₂O₄)]·H₂O, abbr. bpV(oxa)} and arginine (abbr. Arg) in solution were studied by 1D multinuclear ( ¹H, ¹³C, ¹⁵N, and ⁵¹V) NMR, 2D diffusion ordered spectroscopy (DOSY), variable temperature NMR, and electrospray ionization mass spectrometry (ESI-MS). Spectroscopic results indicated that a new peroxovanadate species [OV(O₂)₂Arg]^- was formed in which Arg coordinates to vanadium through amino group. It is proved that these methods are useful for analyzing and characterizing the reaction processes and coordination modes in this kind of the interaction systems.

Key words: peroxovanadate, arginine, interaction, NMR, DOSY, ESI-MS

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ZENG Bi-Rong, YU Xian-Yong, CAI Shu-Hui, CHEN Zhong, WAN Hui-Lin. NMR Studies on Interactions between Oxalate-oxodiperoxovanadate and Arginine[J]. Acta Chimica Sinica, 2004, 62(3): 230-235.

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NMR研究草酸双过氧钒配合物与精氨酸的相互作用

NMR Studies on Interactions between Oxalate-oxodiperoxovanadate and Arginine

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