Research Progress of Covalent Organic Framework Materials in Catalysis

doi:10.6023/A19120426

Acta Chimica Sinica ›› 2020, Vol. 78 ›› Issue (4): 311-325.DOI: 10.6023/A19120426 Previous Articles Next Articles

Special Issue: 多孔材料：共价有机框架(COF)

Review

共价有机框架材料催化研究进展

刘建国^a,b,c, 张明月^a,b, 王楠^a,b,d, 王晨光^a,b, 马隆龙^a,b,d

a 中国科学院广州能源研究所中国科学院可再生能源重点实验室广州 510640;
b 中国科学院大学北京 100049;
c 中国科学院洁净能源创新院大连 116023;
d 天津大学环境科学与工程学院天津 300350

投稿日期:2019-12-14 发布日期:2020-04-09
通讯作者: 刘建国, 马隆龙 E-mail:liujg@ms.giec.ac.cn;mall@ms.giec.ac.cn
作者简介:刘建国,男,中国科学院广州能源研究所研究员.2017年在瑞典斯德哥尔摩大学获得有机化学博士学位.随后在瑞典中部大学、新加坡国立大学、乌普萨拉大学从事博士后研究.2018年起担任中国科学院广州能源研究所研究员.主要研究方向包括催化化学、生物质精细化工、有机金属催化等交叉学科领域;张明月,男,中国科学院广州能源研究所在读研究生.2019年于辽宁科技大学能源与动力工程系获工学学士学位.主要从事生物质精细化工品制备以及生物质平台分子高值化合成药物中间体研究;王楠,女,天津大学在读博士研究生.2015年于厦门大学化学化工学院获工学硕士学位.目前研究方向为新型纳米催化材料的制备及其在生物质精细化工的应用;王晨光,男,中国科学院广州能源研究所研究员.2009年毕业于中国科学院广州能源研究所,获得热能工程专业博士学位.2009～2010年赴美国明尼苏达大学作为博士后开展海藻的超临界转化研究,2010～2013年于科罗拉多矿业大学作为博士后开展生物质基燃料燃烧热解特性研究,2013年9月起担任中国科学院广州能源研究所研究员、博士生导师.研究内容涉及生物质热解,生物质气的净化重整,气相化学机理,生物质基燃料模拟燃烧,基于生物质定向转化的催化新技术等;马隆龙,男,博士,中国科学院广州能源研究所研究员,博士生导师,973项目首席科学家.1994年至1995年在意大利ENEA Trisaia研究中心做高级访问学者.“十二五” 863计划“农林生物质高效转化技术”主题专家组专家,“十三五”国家重点研发计划“可再生能源与氢能重点专项”专家组专家,生物质能源产业技术创新战略联盟理事长,国家能源生物燃料中心主任,中国可再生能源学会生物质能专业委员会副主任委员.主要研究方向为生物质高效转化与综合利用,包括:(1)生物水相催化转化理论基础研究,(2)生物质热解、气化及发电,(3)生物质全组分高效转化与利用.
基金资助:
项目受国家自然科学基金面上项目（No.51976225）和中国科学院洁净能源创新研究院合作基金项目（No.DNL201916）资助.

Research Progress of Covalent Organic Framework Materials in Catalysis

Liu Jianguo^a,b,c, Zhang Mingyue^a,b, Wang Nan^a,b,d, Wang Chenguang^a,b, Ma Longlong^a,b,d

a Key Laboratory of Renewable Energy, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, China;
b University of Chinese Academy of Sciences, Beijing 100049, China;
c Dalian National Laboratory for Clean Energy, Dalian 116023, China;
d School of Environmental Science and Engineering, Tianjin University, Tianjin 300350, China

Received:2019-12-14 Published:2020-04-09
Supported by:
Project supported by the National Natural Science Foundation of China (No. 51976225) and Dalian National Laboratory for Clean Energy Cooperation Fund, Chinese Academy of Sciences (No. DNL201916).

Covalent organic framework materials (COFs) are a class of organic porous materials with large specific surface area, high porosity and crystallinity. Owning to their special nature of functional versatility and easy modification, COFs can be designed to be efficient catalysts either embed functional active sites into the skeleton through a "top-down" strategy, or load metal nanoparticles into the framework via a post-modification approach. These studies have laid the foundation for the extension of COF's application in heterogeneous and other catalytic fields. The synthetic strategy and application of COF in different types of catalytic reactions are reviewed in this paper. Moreover, the current research situation of COF catalyst is summarized and prospected. Finally, the remaining challenges in this field are also indicated.

Key words: covalent organic framework, porous material, COF supporter, catalyst, heterogeneous catalysis

Cite this article

Liu Jianguo, Zhang Mingyue, Wang Nan, Wang Chenguang, Ma Longlong. Research Progress of Covalent Organic Framework Materials in Catalysis[J]. Acta Chimica Sinica, 2020, 78(4): 311-325.

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共价有机框架材料催化研究进展

Research Progress of Covalent Organic Framework Materials in Catalysis

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