CO2捕集分离的功能离子液体及材料研究进展★

doi:10.6023/A23030063

化学学报 ›› 2023, Vol. 81 ›› Issue (6): 627-645.DOI: 10.6023/A23030063 上一篇下一篇

所属专题：庆祝《化学学报》创刊90周年合辑

综述

CO₂捕集分离的功能离子液体及材料研究进展^★

曾少娟, 孙雪琦, 白银鸽, 白璐, 郑爽, 张香平, 张锁江^*()

中国科学院过程工程研究所多相复杂系统国家重点实验室离子液体清洁过程北京市重点实验室北京 100190

投稿日期:2023-03-03 发布日期:2023-04-26

作者简介:

曾少娟, 2007年在东华大学获硕士学位, 同年进入中国科学院过程工程研究所工作, 2016年获中国科学院过程工程研究所博士学位, 现为中国科学院过程工程研究所研究员. 主要研究方向: 离子液体构效关系、功能离子液体/材料设计合成和气体分离应用.

张锁江, 1986年获河南大学学士学位; 1994年获浙江大学博士学位, 之后进入北京化工大学做博士后; 1995年获得日本文部省奖学金在日本留学; 2001年回国进入中国科学院过程工程研究所工作, 2010年任中国科学院过程工程研究所所长, 2015年当选为中国科学院院士. 主要研究方向: 离子液体与绿色过程, 包括离子液体的分子设计、规模制备和清洁工艺.

^★庆祝《化学学报》创刊90周年.

基金资助:
国家重点研发计划(2022YFB4101701); 国家自然科学基金(22122814); 国家自然科学基金(21890764); 中国科学院青年创新促进会(2018064)

Research Progress of CO₂ Capture and Separation by Functionalized Ionic Liquids and Materials^★

Shaojuan Zeng, Xueqi Sun, Yinge Bai, Lu Bai, Shuang Zheng, Xiangping Zhang, Suojiang Zhang()

Beijing Key Laboratory of Ionic Liquids Clean Process, State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190

Received:2023-03-03 Published:2023-04-26
Contact: * E-mail: sjzhang@ipe.ac.cn
About author:
^★Dedicated to the 90th anniversary of Acta Chimica Sinica.
Supported by:
National Key R&D Program of China(2022YFB4101701); National Natural Science Foundation of China(22122814); National Natural Science Foundation of China(21890764); Youth Innovation Promotion Association of the Chinese Academy of Sciences(2018064)

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摘要/Abstract

CO₂排放是一个严峻的全球性问题, 要实现我国双碳战略目标, CO₂捕集技术不可或缺. 离子液体作为一类新型分离介质, 因其特有的低挥发性、良好的气体溶解性和结构可设计性等优势, 在CO₂捕集分离领域备受关注. 重点讨论了近五年来所报道的氨基和非氨基功能离子液体、离子液体复配溶剂、离子液体杂化吸附和膜材料在CO₂捕集分离方面的研究进展, 总结了氨基、电负性等功能位点对CO₂分离性能及机理的影响规律, 以及功能离子液体在复配溶剂、吸附和膜材料中发挥的作用, 并对离子液体法CO₂捕集技术的未来发展方向和前景提出了展望.

关键词: 离子液体, CO₂捕集, 吸收, 吸附, 膜分离

CO₂ emission is a serious global problem. CO₂ capture technology is indispensable to achieve the strategic goals of carbon peaking and carbon neutrality in China. Ionic liquids as new media have attracted much attention in the field of CO₂ capture and separation due to their unique advantages of low volatility, good gas solubility and structure designability. This review focuses on research progresses of amino and non-amino functionalized ionic liquids, ionic liquid hybrid solvents, ionic liquid modified adsorbents and membranes for CO₂ capture and separation reported in the past five years. The influence of amino groups and electronegative functional sites on CO₂ separation performance and mechanism, and the role of functionalized ionic liquids in hybrid solvents, adsorbents and membranes were summarized. Finally, the future development direction and prospect of ionic liquid-based CO₂ capture technologies were also proposed.

Key words: ionic liquids, CO₂ capture, absorption, adsorption, membrane separation

引用此文

曾少娟, 孙雪琦, 白银鸽, 白璐, 郑爽, 张香平, 张锁江. CO₂捕集分离的功能离子液体及材料研究进展^★[J]. 化学学报, 2023, 81(6): 627-645.

Shaojuan Zeng, Xueqi Sun, Yinge Bai, Lu Bai, Shuang Zheng, Xiangping Zhang, Suojiang Zhang. Research Progress of CO₂ Capture and Separation by Functionalized Ionic Liquids and Materials^★[J]. Acta Chimica Sinica, 2023, 81(6): 627-645.

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图/表 20

图1. 用于CO2捕集的代表性功能阴离子(a)和阳离子(b)结构

Figure 1. The structures of functionalized anions (a) and cations (b) for CO2 capture

图2. [NH2p-bim][BF4]与CO2的反应机理[8]

Figure 2. Proposed reaction mechanism of CO2 with [NH2p-bim][BF4][8]

图3. H2S和CO2与叔氨基功能离子液体的反应机理[11]

Figure 3. Reaction mechanisms of H2S and CO2 with tertiary-amine functionalized ionic liquids[11]

图4. [DMEDAH][formate]与CO2可能反应路径[13]

Figure 4. Possible reaction pathways between [DMEDAH][formate] and CO2[13]

图5. CO2与[P66614][Met](上)和[P66614][Pro](下)的反应示意图[16]

Figure 5. Reaction diagram of CO2 with [P66614][Met] (top) and [P66614][Pro] (bottom)[16]

图6. [N66614][Lys]与CO2的反应路径[19a]

Figure 6. The reaction pathway for [N66614][Lys] and CO2[19a]

图7. [IDA]-和[Gly]-阴离子与CO2之间的多位点作用[19c]

Figure 7. Multiple-site interaction of [IDA]- and [Gly]- with CO2[19c]

图8. 氨基酸离子液体吸收CO2的可能路径[21]

Figure 8. Possible CO2 absorption pathways in amino acid ionic liquid[21]

图9. 氨基酸离子液体吸收CO2的反应机制[23]

Figure 9. Reaction mechanism of CO2 absorption by amino acid ionic liquid[23]

图10. [Gly]-(a)和 [aN111]＋(b)有水和无水条件下CO2反应路径[28]

Figure 10. CO2 absorption energies of [Gly]- (a) and [aN111]＋(b) in the presence and absence of water[28]

图11. [APmim][Lys]水溶液吸收CO2的反应机理[29a]

Figure 11. Reaction mechanism of CO2 capture in [APmim][Lys] solution[29a]

图12. [DCP5]-与CO2之间的多位点作用[37]

Figure 12. Multiple-site interactions between the [DCP5]- and CO2[37]

图13. [P4442][Cy-Suc]多位点协同吸收CO2的机理[45]

Figure 13. CO2 absorption mechanism by [P4442][Cy-Suc] through multiple-site cooperative interactions[45]

图14. [TMGH][Im]和[TMGH][Im]-H2O体系的CO2吸收途径[57]

Figure 14. CO2 absorption pathways of [TMGH][Im] and [TMGH][Im]-H2O systems[57]

图15. [Apmim][BF4]-MEA-DEEA-H2O协同强化CO2捕集机理[62]

Figure 15. Co-enhancement mechanism of CO2 capture by [Apmim][BF4]-MEA-DEEA-H2O[62]

图16. [TEPAH][AICA]/NPA/EG溶液的CO2捕获机制

Figure 16. CO2 capture mechanism of the [TEPAH][AICA]/NPA/EG solution AFILN represented the N atom of [AICA]?; AFILT, AFILM and AFILA represented the amino groups of [TEPAH]＋, imidazole ring and amide, respectively.[69]

图17. CO2与[MEAH][Im]-EG (1∶3)的反应[75]

Figure 17. The reaction between CO2 and [MEAH][Im]-EG (1∶3)[75]

图18. DBN-[Bmim]Cl-Im (1∶1∶1)与CO2之间的可能机理[77]

Figure 18. Plausible mechanism between DBN-[Bmim]Cl-Im (1∶1∶1) and CO2[77]

图19. 多孔离子液体UIO-66-liquid/[M2070][IPA]的构筑原理及对CO2吸附过程[98]

Figure 19. Construction principle and CO2 adsorption process of porous ionic liquid UIO-66-liquid/[M2070][IPA][98]

图20. TSIL@NH2-MIL-101(Cr)/PIM-1膜分离CO2[109]

Figure 20. TSIL@NH2-MIL-101(Cr)/PIM-1 membrane for CO2 separation[109]

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CO₂捕集分离的功能离子液体及材料研究进展^★

Research Progress of CO₂ Capture and Separation by Functionalized Ionic Liquids and Materials^★

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