Advance and Prospective on CO2 Activation and Transformation Strategy

doi:10.6023/cjoc202004030

Abstract

Climate change and depletion of fossil fuels have drawn considerable attention. Considering carbon dioxide is both the dominant greenhouse gas and renewable C₁ source, CO₂ valorization into valuable chemicals is considered to reconcile the environment benefit and sustainable chemistry development. Unfortunately, the thermodynamic stability and kinetic inertness of CO₂ make its chemical transformation challenging. As a consequence, developing highly efficient catalytic systems and synthetic protocols is crucial for CO₂ conversion. In recent years, He's group made great progress on strategy design and catalyst development for CO₂ conversion. A series novel CO₂ conversion strategies are proposed, including CO₂ capture and in-situ transformation, hierarchical reductive functionalization of CO₂, designing thermodynamically favorable reactions by multi-component cascade reaction and photo-promoted CO₂ transformation. Concurrently, the corresponding highly efficient catalytic systems were also developed based on the reaction mechanism and thus CO₂ transformation was successfully performed under mild conditions. It is hoped that this review can arouse broad concern on CO₂ transformation and spur its further development.

Key words: carbon dioxide, capture, transformation, reduction, cascade reaction, photocatalysis, sustainable chemistry, synthetic method

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Chen Kaihong, Li Hongru, He Liangnian. Advance and Prospective on CO₂ Activation and Transformation Strategy[J]. Chinese Journal of Organic Chemistry, 2020, 40(8): 2195-2207.

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CO₂活化和转化策略研究进展

Advance and Prospective on CO₂ Activation and Transformation Strategy

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[15]	Ning Chen, Chengdong Zhang, Peng Li, Ge Qiu, Yinjie Liu, Tianlei Zhang. Research Progress in Synthesis of Spirocyclic Compounds Driven by Photo/Electrochemistry [J]. Chinese Journal of Organic Chemistry, 2023, 43(7): 2293-2303.

CO2活化和转化策略研究进展